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A kind of phosphate modified attapulgite magnetic passivation agent and using method thereof

A technology of attapulgite and phosphate, applied in chemical instruments and methods, land preparation methods, applications, etc., can solve problems such as cumbersome process and secondary pollution, achieve increased specific surface area, improved passivation effect, and improved surface adsorption points Effect

Active Publication Date: 2021-07-30
浙江正峰生态环境工程有限公司
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

Yin Zhigang et al. (invention patent 201910554538.X) proposed a porous magnetic material and its preparation method, using a magnetic passivator to completely remove heavy metals, but the process is cumbersome; Wang Yangyang et al. (invention patent 201910226818.8) also proposed a Highly magnetically modified biochar and its preparation method and its application in the treatment of heavy metal pollution in soil. This method utilizes the biochar carrier modification method to prepare a magnetic passivator, but this method introduces dimethyl Sodium dithiocarbamate solution, there may be secondary pollution problems

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0028] 1) Preparation of phosphate-modified attapulgite: Weigh 3g parts by weight of trisodium phosphate into a container, add an appropriate amount of deionized water, stir for 25 minutes, add 7g parts by weight of attapulgite, and add deionized water to make the water-to-soil weight ratio 18 : 0.5, ultrasonic vibration for 8h, standing for 25min, suction filtration, the obtained filter residue was repeatedly rinsed with deionized water, dried, and ground through a 120 mesh sieve to obtain phosphate modified attapulgite powder;

[0029] 2) Material magnetization:

[0030] a. Add deionized water in the container, then add 0.7g parts by weight of phosphate modified attapulgite, 5g parts by weight of FeCl 3 ▪6H 2 O and 2g parts by weight FeSO 4 ▪7H 2 O, phosphate-modified attapulgite: the weight-to-volume ratio of deionized water is 170ml: 0.7g, heated in a nitrogen environment at 65°C;

[0031] b. Add 7mol / L NaOH solution dropwise, the volume ratio of NaOH solution: deioniz...

Embodiment 2

[0034] 1) Weigh 3.929g of trisodium phosphate into a beaker, add an appropriate amount of deionized water, stir for 30 minutes, add 10g of attapulgite, add deionized water to keep the water-soil ratio at 20:1, ultrasonically shake for 10h, stand for 30min, and filter with suction , the obtained filter residue is repeatedly washed with deionized water, dried, and ground through a 100-mesh sieve to obtain a phosphate-modified attapulgite powder;

[0035] 2) Material magnetization:

[0036] a. Add 200ml deionized water to a 500ml beaker, then add 1.0g phosphate modified attapulgite and 5.96g FeCl 3 ▪6H 2 O, 3.06 g FeSO 4 ▪7H 2 O, heated in a nitrogen atmosphere at 70°C;

[0037] b. Add 10ml of 8.0mol / L NaOH solution dropwise to precipitate iron oxide in the solution, adjust the pH to 11.0, stir for 1h, age the mixture at 70°C for 4h, wash with double deionized water until the supernatant is medium The obtained material is baked at 100°C for 3 hours, and ground through a 100-...

Embodiment 3

[0040] 1) Preparation of phosphate-modified attapulgite: Weigh 5g of trisodium phosphate into a container, add an appropriate amount of deionized water, stir for 35 minutes, add 13g of attapulgite, add deionized water to make the water-soil weight ratio 22:1.5, and ultrasonically Shaking for 12 hours, standing still for 35 minutes, and suction filtering, the resulting filter residue was repeatedly washed with deionized water, dried, and ground through an 80-mesh sieve to obtain phosphate-modified attapulgite powder;

[0041] 2) Material magnetization:

[0042] a. Add deionized water to the container, then add 1.3g phosphate modified attapulgite, 7g FeCl 3 ▪6H 2 O and 4gFeSO 4 ▪7H 2 O, phosphate-modified attapulgite: the weight-to-volume ratio of deionized water is 230ml: 1.3g, heated in a nitrogen environment at 75°C;

[0043] b. Add 9mol / L NaOH solution dropwise, the volume ratio of NaOH solution: deionized water is 1.2ml: 23ml, precipitate the iron oxide in the solution,...

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PUM

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Abstract

A phosphate-modified attapulgite magnetic passivator and a use method thereof belong to the technical field of moderately and lightly polluted farmland restoration. The following methods are used to prepare: 1) preparation of phosphate modified attapulgite; 2) material magnetization; 3) magnetization inspection. The above-mentioned phosphate-modified attapulgite magnetic passivator and its use method, through the modification method, on the basis of the original adsorption, complexation, precipitation, and ion exchange of the passivator, the passivator is given magnetic properties, and the preparation Finally, the heavy metals are completely removed from the soil by magnetic separation, and the total amount of lead and cadmium in the farmland soil is significantly reduced, which meets the restoration requirements and has broad application prospects.

Description

technical field [0001] The invention belongs to the technical field of moderately and lightly polluted farmland restoration, and specifically relates to a phosphate-modified attapulgite magnetic passivator and a use method thereof. Background technique [0002] Due to the stable nature of heavy metals, it is difficult to be degraded by microorganisms, and they are easy to accumulate in the soil and cause soil heavy metal pollution. Heavy metal pollution in agricultural land soil is closely related to human life. Heavy metals in soil can enter the human body through the food chain, which poses a great threat to human health. According to the 2014 National Soil Pollution Survey Bulletin, my country's agricultural land soil is seriously polluted by heavy metals, and the rate of soil points exceeding the standard in cultivated land, forest land, and grassland is as high as 19.4%, 10.0%, and 10.4%, respectively. Soil pollution needs to be repaired urgently. [0003] Farmland soi...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C09K17/08A01B79/00C09K101/00
CPCA01B79/00C09K17/08C09K2101/00
Inventor 劳千峰
Owner 浙江正峰生态环境工程有限公司