Unlock instant, AI-driven research and patent intelligence for your innovation.

A processing technology for improving the quality of activated carbon through sulfuric acid pretreatment

A processing technology, activated carbon technology, applied in the direction of carbon compounds, inorganic chemistry, chemical instruments and methods, etc., can solve the problems of impaired activated carbon quality, reduced activated carbon yield, low activation temperature, etc., to improve quality and inhibit phenolic substances The effect of generation and specific surface area improvement

Active Publication Date: 2021-09-24
NANJING FORESTRY UNIV
View PDF0 Cites 0 Cited by
  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0002] Lignin is the second largest natural polymer in nature. Lignin has the characteristics of renewable, wide sources, low price, abundant reserves and environmental friendliness. It can be applied in a wide range of fields, and lignin consists of phenylpropane structure The units are connected by carbon-carbon bonds and ether bonds, and the carbon content is high, so it is suitable as a raw material for the production of activated carbon. At present, activated carbon produced by the phosphoric acid method of wood raw materials is widely used in the field of liquid phase adsorption. Compared with other activated carbon preparation methods, this Activated carbon by phosphoric acid method has the advantages of low activation temperature, short activation time and high product yield. Activated carbon by phosphoric acid method is characterized by well-developed mesopores and a specific surface area of ​​900-1300m2 / g, and the production process of activated carbon by phosphoric acid method is very mature. Optimization has been difficult to further improve the quality of phosphoric acid-based activated carbon. There are hydroxyl groups, methoxy groups and other groups on the phenylpropane in lignin, which improves the activity of lignin decomposition, which will occur before lignin reaches the activation temperature. Violent decomposition produces by-products such as tar, which reduces the yield of activated carbon and hinders the quality of activated carbon

Method used

the structure of the environmentally friendly knitted fabric provided by the present invention; figure 2 Flow chart of the yarn wrapping machine for environmentally friendly knitted fabrics and storage devices; image 3 Is the parameter map of the yarn covering machine
View more

Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0039] Fully mix lignin with 5% sulfuric acid solution, the mass ratio of lignin to sulfuric acid solution is 1:1, place in a tube furnace, heat up to 180°C at a heating rate of 5°C / min, and keep at this temperature 30min, obtained product A;

[0040] Take the product A obtained in the previous step and add an activator 30% phosphoric acid solution to fully infiltrate and mix evenly, the product A:activator mass ratio is 1:1, and the product B is obtained;

[0041] The product B obtained in the previous step was placed in a tube furnace, and under the protection of nitrogen or other inert gases, the temperature was raised to 525 ° C at a heating rate of 2 ° C / min, and the product C was obtained by keeping it warm for 30 minutes;

[0042] The product C obtained in the previous step was cooled to room temperature under the protection of nitrogen, washed with deionized water until neutral, and finally dried in an oven at 100°C for 3 hours to prepare activated carbon.

Embodiment 2

[0044] Fully mix lignin with 12% sulfuric acid solution, the mass ratio of lignin to sulfuric acid solution is 1:1, place in a tube furnace, heat up to 190°C at a heating rate of 12°C / min, and keep at this temperature 75min, obtained product A;

[0045] Take the product A obtained in the previous step and add the activator 45% phosphoric acid solution to fully infiltrate and mix evenly, the product A:activator mass ratio is 2:5, and the product B is obtained;

[0046] Take the product B obtained in the previous step and place it in a tube furnace, under the protection of nitrogen or other inert gas, raise the temperature to 550°C at a heating rate of 6°C / min, keep it warm and activate for 60min, and obtain product C;

[0047]The product C obtained in the previous step was cooled to room temperature under the protection of nitrogen, washed with deionized water until neutral, and finally dried in an oven at 105°C for 4 hours to prepare activated carbon.

Embodiment 3

[0049] Fully mix lignin with 20% sulfuric acid solution, the mass ratio of lignin to sulfuric acid solution is 1:1, place in a tube furnace, heat up to 200°C at a heating rate of 20°C / min, and keep at this temperature 120min, obtained product A;

[0050] Take the product A obtained in the previous step and add the activator 60% phosphoric acid solution to fully infiltrate and mix evenly, the product A:activator mass ratio is 1:4, and the product B is obtained;

[0051] The product B obtained in the previous step was placed in a tube furnace, and under the protection of nitrogen or other inert gases, the temperature was raised to 575°C at a heating rate of 10°C / min, and the product C was obtained by keeping it warm for 90 minutes;

[0052] The product C obtained in the previous step was cooled to room temperature under the protection of nitrogen, washed with deionized water until neutral, and finally dried in an oven at 110°C for 5 hours to prepare activated carbon.

the structure of the environmentally friendly knitted fabric provided by the present invention; figure 2 Flow chart of the yarn wrapping machine for environmentally friendly knitted fabrics and storage devices; image 3 Is the parameter map of the yarn covering machine
Login to View More

PUM

PropertyMeasurementUnit
specific surface areaaaaaaaaaaa
Login to View More

Abstract

The invention discloses a processing technology for improving the quality of activated carbon through sulfuric acid pretreatment, which comprises the following steps: 1) acid treatment; 2) mixing; 3) preparation; 4) cleaning. The invention prepares activated carbon by using enzymatic lignin as raw material to realize the added value utilization of enzymatic lignin, pretreat lignin with sulfuric acid, make it dehydrate and condense at a lower temperature, realize lignin polymerization, and inhibit The production of phenolic substances increases the degree of polymerization of lignin, and the specific surface area of ​​activated carbon obtained after activation is significantly increased, the yield of activated carbon is increased, and the quality of activated carbon is improved, which is suitable for widespread promotion and use.

Description

technical field [0001] The invention relates to the field of activated carbon processing, in particular to a processing technology for improving the quality of activated carbon through sulfuric acid pretreatment. Background technique [0002] Lignin is the second largest natural polymer in nature. Lignin has the characteristics of renewable, wide sources, low price, abundant reserves and environmental friendliness. It can be applied in a wide range of fields, and lignin consists of phenylpropane structure The units are connected by carbon-carbon bonds and ether bonds, and the carbon content is high, so it is suitable as a raw material for the production of activated carbon. At present, activated carbon produced by the phosphoric acid method of wood raw materials is widely used in the field of liquid phase adsorption. Compared with other activated carbon preparation methods, this Activated carbon by phosphoric acid method has the advantages of low activation temperature, shor...

Claims

the structure of the environmentally friendly knitted fabric provided by the present invention; figure 2 Flow chart of the yarn wrapping machine for environmentally friendly knitted fabrics and storage devices; image 3 Is the parameter map of the yarn covering machine
Login to View More

Application Information

Patent Timeline
no application Login to View More
Patent Type & Authority Patents(China)
IPC IPC(8): C01B32/342C01B32/324
CPCC01B32/324C01B32/342
Inventor 陈登宇章捷马欢欢周建斌章一蒙王恋
Owner NANJING FORESTRY UNIV