Acid-curable, refractory particulate material composition for forming mold
A technology of granular materials and compositions, applied in the direction of casting molds, casting molding equipment, cores, etc., can solve the problems that the strength of casting molds needs to be further improved
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Embodiment 1
[0040] Synthesis Example 1: Synthesis of polycondensation product of furfuryl alcohol-phenol-formaldehyde (phenol-modified furan resin)
[0041]Add 975 parts (10.4 moles) of phenol and 18 parts (0.16 moles) of 48.5% potassium hydroxide aqueous solution to a four-necked flask equipped with a thermometer, a condenser and a stirrer, and add at a constant temperature of 80°C for about 1 hour 507 parts (15.5 moles) of 92% paraformaldehyde. Keep at a constant temperature of 80° C. for 6 hours, then cool rapidly and adjust its pH value to 5.0 by neutralizing with 50% sulfuric acid. After neutralization, centrifuge Isolate the neutralized salt. Add 1500 parts of furfuryl alcohol to the obtained resin, and then add 0.3 parts of N-β-(aminoethyl)-γ-aminopropylmethyldimethoxysilane to obtain phenol-modified Furan resin composition.
Embodiment 2
[0042] Synthesis Example 2: Synthesis of phenol-formaldehyde polycondensation product (phenolic resin)
[0043] Add 1950 parts (20.7 moles) of phenol and 36 parts (0.31 moles) of 48.5% potassium hydroxide aqueous solution to a four-necked flask equipped with a thermometer, condenser and stirrer, and add at a constant temperature of 80°C for about 1 hour 1014 parts (31.1 moles) of 92% paraformaldehyde. When the viscosity of the system reaches 30,000 centipoise at 25°C, it is rapidly cooled and neutralized with 50% sulfuric acid until the pH value reaches 5.0. After neutralization, centrifuge Separate the neutralized salt. Add water to it until its water content reaches 20%, and then add 0.3 parts of N-β-(aminoethyl)-γ-aminopropylmethyldimethoxysilane to obtain a phenolic resin combination thing.
Embodiment 3
[0044] Synthesis Example 3: Synthesis of furfuryl alcohol-urea-formaldehyde polycondensation product (urea-modified furan resin)
[0045] Add 682.4 parts (6.96 moles) of furfuryl alcohol, 85.7 parts (1.43 moles) of urea, 231.9 parts (2.86 moles) of 37% formaldehyde and 0.08 parts of 25% hydroxide to a four-necked flask equipped with a thermometer, condenser and stirrer Sodium aqueous solution, the mixture was further reacted at 100°C for 1 hour. Thereafter, 0.2 parts of 10% hydrochloric acid was added thereto, followed by further reaction at 100°C for 3 hours. 0.3 parts of N-β-(aminoethyl)-γ were added thereto -Aminopropylmethyldimethoxysilane to obtain a urea-modified furan resin composition.
[0046] According to the present invention, the acid-hardening resin composition thus obtained is used to prepare a granular composition for casting to form a casting mold. If a solvent needs to be added, it is added to the above-prepared resin composition and mixed with it.
[0047]...
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