Amorphous substance of 17alpha-acetoxy-11beta-(4-N,N-dimethylaminophenyl)-19-norpregn-4,9-diene-3,20-diketone and preparation method thereof
A technology of dimethylaminophenyl and norpregnant, which is applied in the directions of steroids, organic chemistry, organic chemistry, etc., can solve the problems of poor thermal stability, not very good stability, low solubility of crystal form A, etc. problems, to achieve the effect of high product purity, scalable operation, and good solubility
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Embodiment 1
[0031] Add 30mL of methanol to 5.0g of CDB-2914 (crystal form A) raw material, heat to 65°C, stir to dissolve the solid completely; after the raw material of CDB-2914 is completely dissolved, slowly add 100ml of water; Stir at 65°C for 4 hours; filter and dry under reduced pressure at 60°C for 12 hours to obtain 4.7g of product with a mass yield of 94% and an HPLC purity of 99.0%.
[0032] Get the amorphous sample of CDB-2914 prepared by the present embodiment, with 1.5460 angstroms wavelength α 1 , 1.54439 Angstroms wavelength α 2 The radiation source, the intensity ratio of α 1 / α 2 The powder X-ray diffraction (XRPD) spectrum that measures in the Dedye-Scherrer INEL CPS-120 equipment of 0.5,40kV voltage and 30mA current intensity is as figure 1 shown by figure 1 It can be seen that the prepared amorphous CDB-2914 does not contain identifiable diffraction peak shapes in the XRPD pattern.
Embodiment 2
[0034] Add 30mL of methanol to 5.0g of CDB-2914 (isopropanol hemisolvate) raw material, heat to 65°C, stir to dissolve the solid completely; after the CDB-2914 raw material is completely dissolved, slowly add 100ml of water; , continue to keep stirring at 65° C. for 4 hours; filter, and dry under reduced pressure at 60° C. for 12 hours to obtain 4.6 g of product with a mass yield of 92% and an HPLC purity of 99.1%.
[0035] The XRPD spectrum of the amorphous matter of CDB-2914 prepared in the present embodiment is as follows: figure 1 shown.
Embodiment 3
[0037] Add 30mL of methanol to 2.0g of CDB-2914 (crystal form A) raw material, heat to 50°C, stir to dissolve the solid completely; after the raw material of CDB-2914 is completely dissolved, slowly add 60ml of water; Stir at 50°C for 3 hours; filter and dry under reduced pressure at 60°C for 12 hours to obtain 1.8 g of product with a mass yield of 90% and an HPLC purity of 99.0%.
[0038] The XRPD spectrum of the amorphous matter of CDB-2914 prepared in the present embodiment is as follows: figure 1 shown.
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