Encapsulates
A mixture and polymer technology, applied in detergent composition, chemical/physical process, organic cleaning composition, etc., can solve the problem of not providing effective encapsulation of solid water-soluble beneficial agent
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[0392] a. Preparation of calibration curve: Add 40 μL of 10.000 ppm detergent in deionized water as described in Examples 7, 8 and 9 to 150 μL of Chicago Sky Blue reagent, and at 37° C. Incubate for 3 minutes (see table below). After incubation, absorbance measurements (Abs 1 ) of the detergent and dye solutions were performed at 600 nm. 60 μL of hydrogen peroxide reagent was added to the solution and incubated at 37° C. for 30 minutes. After incubation, the absorbance (Abs 2) of the solution was measured at 600 nm. Repeat the protocol with different levels of metal catalyst according to the table below:
[0393] sample
Xppm metal catalyst
Abs 1
Abs 2
ABS=Abs 1-Abs 2
0
0
1
0.05
2
0.10
3
0.20
4
0.30
5
0.40
6
0.50
7
...
Embodiment 1
[0414] Example 1: Preparation of encapsulates by interfacial polymerization
[0415] Core preparation: 40 g of the suspension composed of a solid water-soluble manganese complex such as meso-5,5,7,12 was cooled to 25°C and mixed with 4.482 g of trimesoyl chloride (Sigma Aldrich). , 12,14-hexamethyl-1,4,8,11-tetraazacyclotetradecane and rac-5,5,7,12,12,14-hexamethyl-1,4,8 , a manganese complex of 11-tetraazacyclotetradecane ligand (99% of the particles have a particle size of 3.65 microns), polysiloxane (60,000 centistokes) and a hydrophobic Sexual organic composition formation. The mixture was kept at 25°C.
[0416] Solution 1 was prepared: 2 grams of polyvinyl alcohol (87-89% hydrolyzed, Mw 13000, Sigma-Aldrich) were dissolved and mixed in 198 grams of deionized water. The solution was cooled to 25°C.
[0417] Solution 2 was prepared: 8.598 grams of diethylenetriamine (Sigma-Aldrich) was mixed with 10 grams of deionized water. The solution was cooled to 25°C.
[0418]...
Embodiment 2
[0420] Example 2: Preparation of encapsulates by thermally induced phase separation
[0421] Preparation of cores: 70 g of a suspension consisting of a solid water-soluble manganese complex such as meso-5,5, 7,12,12,14-Hexamethyl-1,4,8,11-Tetraazacyclotetradecane and rac-5,5,7,12,12,14-Hexamethyl-1, Manganese complex of 4,8,11-tetraazacyclotetradecane ligand (99% of the particles have a particle size of 3.65 microns), polysiloxane (60,000 centistokes) and materials listed in Tables 1 to 10 A formulated hydrophobic organic composition is formed. The mixture was kept at 5°C.
[0422] Prepare Solution 1: Dissolve 1.8 g of polyvinyl alcohol at 60 °C 70-75 (DuPont) was dissolved in 148.2 grams of deionized water. The solution was cooled to 5°C.
[0423] Solution 2 was prepared: 1.87 grams of hydroxypropylmethylcellulose (Sigma-Aldrich) was dissolved in 60 grams of deionized water. The solution was kept at 5°C until the hydroxypropylmethylcellulose was completely dissolved....
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