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A kind of antibacterial hydrogel material and preparation method thereof

A technology of hydrogel and glycidyl ester, applied in botany equipment and methods, fungicides, chemicals for biological control, etc., can solve the problems of short antibacterial validity period, easy leakage of antibacterial agents, unstable antibacterial effect, etc.

Active Publication Date: 2021-07-23
CHANGCHUN INST OF APPLIED CHEMISTRY - CHINESE ACAD OF SCI
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0005] The above-mentioned hydrogel materials are all endowed with antibacterial properties by blending and doping substances with antibacterial functions. The materials prepared by this method are release-type antibacterial materials, which generally have the characteristics of easy leakage of antibacterial agents, unstable antibacterial effect, and Disadvantages of short antibacterial validity period

Method used

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Examples

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preparation example Construction

[0025] The invention provides a kind of preparation method of antibacterial hydrogel material, comprises the following steps:

[0026] A) under the action of catalyst, polyvinyl alcohol solution is reacted with glycidyl methacrylate to obtain functionalized polyvinyl alcohol;

[0027] B) Copolymerize and cross-link the functionalized polyvinyl alcohol aqueous solution and methacryloyloxyethyltrimethylammonium chloride under the condition of an initiator to obtain an antibacterial hydrogel material.

[0028] In the invention, under the action of a catalyst, the polyvinyl alcohol solution is reacted with glycidyl methacrylate to obtain functionalized polyvinyl alcohol. Specifically, it may be: add a catalyst to the polyvinyl alcohol solution, stir and mix, and then add glycidyl methacrylate for reaction to obtain functionalized polyvinyl alcohol.

[0029] In an embodiment of the present invention, the catalyst includes triethanolamine.

[0030] In some embodiments of the prese...

Embodiment 1

[0055] Add 10 mL of dimethyl sulfoxide and 1 g of polyvinyl alcohol into a 100 mL two-necked flask, heat at 100°C for 3 hours, then add 50 μL of triethanolamine and cool down to 90°C, continue stirring for 1 hour, then add 100 μL of glycidyl methacrylate, and react for 2 hours After cooling down to room temperature, the product is precipitated in acetone, and the product is functionalized polyvinyl alcohol.

[0056] Add 10 mL of deionized water into a 100 mL two-necked flask, add 0.5 g of functionalized polyvinyl alcohol, and heat at 100°C for 3 hours to obtain an aqueous solution of functionalized polyvinyl alcohol;

[0057] The aqueous solution of the functionalized polyvinyl alcohol was transferred to a dialysis bag with a molecular weight cut-off of 3000, dialyzed in deionized water for 24h, and then added 0.25g methacryloyloxyethyl trimethyl ammonium chloride ( DMC), 10 mL of dialyzed functionalized polyvinyl alcohol aqueous solution, fully dissolved in an ice bath under ...

Embodiment 2

[0062] Add 10 mL of dimethyl sulfoxide and 1 g of polyvinyl alcohol into a 100 mL two-necked flask, heat at 100°C for 3 hours, then add 50 μL of triethanolamine and cool down to 90°C, continue stirring for 1 hour, then add 100 μL of glycidyl methacrylate, and react for 2 hours After cooling down to room temperature, the product is precipitated in acetone, and the product is functionalized polyvinyl alcohol.

[0063] Add 10 mL of deionized water into a 100 mL two-necked flask, add 0.5 g of functionalized polyvinyl alcohol, and heat at 100°C for 3 hours to obtain an aqueous solution of functionalized polyvinyl alcohol;

[0064] The aqueous solution of the functionalized polyvinyl alcohol was transferred to a dialysis bag with a molecular weight cut-off of 3000, dialyzed in deionized water for 24h, and then added 0.5g methacryloyloxyethyl trimethyl ammonium chloride ( DMC), 10 mL of dialyzed functionalized polyvinyl alcohol aqueous solution, fully dissolved in an ice bath under a...

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Abstract

The invention relates to the technical field of organic synthesis, in particular to an antibacterial hydrogel material and a preparation method thereof. The preparation method of the antibacterial hydrogel material comprises: A) under the action of a catalyst, polyvinyl alcohol solution reacts with glycidyl methacrylate to obtain functionalized polyvinyl alcohol; B) under the condition of an initiator , the functionalized polyvinyl alcohol aqueous solution and methacryloyloxyethyltrimethylammonium chloride are copolymerized and cross-linked to obtain an antibacterial hydrogel material. The present invention firstly prepares functionalized polyvinyl alcohol, and then, under the action of an initiator, carries out copolymerization and crosslinking of the aqueous solution of the functionalized polyvinyl alcohol and methacryloyloxyethyltrimethylammonium chloride, Thus the antibacterial hydrogel material is prepared. The antibacterial hydrogel material prepared by the preparation method of the present invention has no antibacterial agent doping, but has better antibacterial effect, and the antibacterial hydrogel material is very stable and difficult to degrade.

Description

technical field [0001] The invention relates to the technical field of organic synthesis, in particular to an antibacterial hydrogel material and a preparation method thereof. Background technique [0002] Hydrogel is a three-dimensional network and can maintain a certain amount of water polymer material, which has the characteristics of viscoelasticity, hydrophilicity, biocompatibility and responsiveness, and can be used as drug delivery, wound dressing, tissue repair and in vivo implantation. Into the wide range of applications such as materials. [0003] Polyvinyl alcohol (PVA) is a synthetic polymer material with good water solubility, low toxicity and excellent biocompatibility. It can be used in contact lenses, film materials, cartilage repair, etc. However, as a biomedical material, pure polyvinyl alcohol has no functions such as antibacterial, anti-adhesion, and promotion of cell proliferation. [0004] Most of the current common hydrogel materials made of polyviny...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C08F261/04C08F220/34C08F8/00C08F16/06A01N25/04A01N37/02A01P3/00A01P1/00
CPCA01N25/04A01N37/02C08F8/00C08F261/04C08F16/06C08F220/34
Inventor 杨旭王宝龙姬相玲沙迪许玖多石凯刘志
Owner CHANGCHUN INST OF APPLIED CHEMISTRY - CHINESE ACAD OF SCI