Pyrazopyrimidinone compounds and use thereof
A kind of technology of pyrazolopyrimidinone and compound, applied in pyrazolopyrimidinone compound and its application field as herbicide, can solve the problem that pyrazolopyrimidinone compound is not disclosed etc.
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[0052] Synthesis of compound 1:
[0053] step 1
[0054]
[0055] Add pyrazolamide (19.0 grams, 0.15 moles) and 100 milliliters of toluene into a 250-ml reaction flask, add oxalyl chloride (5 grams, 0.03 moles) and stir at room temperature until no gas is released, slowly heat up to reflux, and react until no gas is released , the solvent was evaporated under reduced pressure, 20 milliliters of o-dichlorobenzene was added to the residue, the temperature was slowly raised until no gas was released, and cooled to room temperature to obtain pyrazolyl isocyanate (5.8 grams, 0.03 mole, yield by 100%) A total of 32 grams of o-dichlorobenzene solution.
[0056] step 2
[0057]
[0058] Add 2-fluoro-4-chloro-5-propargyloxyaniline (1.0 g, 0.005 mol) and 10 ml of toluene into a 50 ml reaction flask, and add pyrazolyl isocyanate (containing o-dichlorobenzene) dropwise under stirring. About 10 grams of the solution, about 0.01 mole, excess), reacted at room temperature for 5 hour...
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