Modified resorcinol phenolic resin and preparation method thereof and rubber compound
A technology of resorcinol phenolic resin and rubber composition, which is applied in the field of modified resorcinol phenolic resin and its preparation, and can solve the problems of reducing resorcinol reactive sites, functional impact, environmental pollution, etc.
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Embodiment 1
[0059] Add 100 parts by mass of resorcinol to a reaction flask equipped with a mechanical stirrer, thermometer, reflux condenser and dropping funnel, heat up to 120°C to melt, add 0.32 parts by mass of p-toluenesulfonic acid monohydrate (Beijing Chemical Reagent Company, purity>98%) were mixed. Add dropwise the 2-allyl phenol of 30 parts by mass (Alfa Aisha (Tianjin) Chemical Co., Ltd., purity > 98%), control the reaction temperature between 120-135 ° C, and drop it in 30 minutes. The reaction was carried out at a temperature of 130° C. for 1 hour. Then, 48 parts by mass of formaldehyde (37% by weight aqueous solution) was slowly added dropwise over 1 hour to perform a reaction. After the dropwise addition of formaldehyde, add 0.3 parts by mass of NaOH aqueous solution (25% by weight) to neutralize, then carry out atmospheric distillation to 150-160°C to remove water and other volatile substances in the reaction system, and obtain a softening point of 120.2 ℃ red resin, free...
Embodiment 2
[0061] Add 100 parts by mass of resorcinol to a reaction flask equipped with a mechanical stirrer, thermometer, reflux condenser and dropping funnel, heat up to 120°C to melt, add 0.32 parts by mass of p-toluenesulfonic acid monohydrate (Beijing Chemical Reagent Company, purity>98%) were mixed. Add dropwise the 2-allyl phenol of 35 parts by mass (Alfa Aisha (Tianjin) Chemical Co., Ltd., purity > 98%), control the reaction temperature between 120-135 ° C, and drop it in 30 minutes. The reaction was carried out at a temperature of 130° C. for 1 hour. Then, 44 parts by mass of formaldehyde (37% by weight aqueous solution) was slowly added dropwise over 1 hour to perform a reaction. After the dropwise addition of formaldehyde, add 0.3 parts by mass of NaOH aqueous solution (25% by weight) to neutralize, then carry out atmospheric distillation to 150-160°C to remove water and other volatile substances in the reaction system, and obtain a softening point of 103.5 ℃ red resin, free...
Embodiment 3
[0063] Add 100 parts by mass of resorcinol to a reaction flask equipped with a mechanical stirrer, thermometer, reflux condenser and dropping funnel, heat up to 120°C to melt, add 0.32 parts by mass of p-toluenesulfonic acid monohydrate (Beijing Chemical Reagent Company, purity>98%) were mixed. Add dropwise the 2-allyl phenol of 40 parts by mass (Alfa Aisha (Tianjin) Chemical Co., Ltd., purity > 98%), control the reaction temperature between 120-135 ° C, and drop it in 30 minutes. The reaction was carried out at a temperature of 130° C. for 1 hour. Then, 44 parts by mass of formaldehyde (37% by weight aqueous solution) was slowly added dropwise over 1 hour to perform a reaction. After the dropwise addition of formaldehyde, add 0.3 parts by mass of NaOH aqueous solution (25% by weight) to neutralize, then carry out atmospheric distillation to 150-160°C to remove water and other volatile substances in the reaction system, and obtain a softening point of 98.4 ℃ red resin, free ...
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