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A kind of phthalocyanine sulfonic acid doped polyaniline anticorrosion coating

A technology of phthalocyanine-based sulfonic acid and anti-corrosion coatings, applied in the field of coatings, can solve the problems of complex, de-doping coating process, and low electrical conductivity, and achieve the effects of simple preparation, good water solubility, and improved electrical conductivity

Active Publication Date: 2016-02-03
四川宇涂科技有限公司
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0007] Aiming at the problems of low electrical conductivity, dedoping phenomenon and complex coating process of existing polyaniline anticorrosion coatings, the present invention provides a phthalocyanine-based coating that effectively overcomes dedoping phenomenon, is simple to prepare, has good adhesion, and has excellent anticorrosion performance. Sulfonic acid doped polyaniline anticorrosion coating

Method used

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Examples

Experimental program
Comparison scheme
Effect test

preparation example Construction

[0021] 3) Preparation of polyaniline anti-corrosion coating: at room temperature, mix phthalocyanine sulfonic acid doped polyaniline, aqueous epoxy resin solution, leveling agent and defoamer, disperse at 1500r / min for 10 minutes, filter Add curing agent and diluent and mix well to get the required anti-corrosion coating; Among them, the viscosity of the water-based epoxy resin solution is 400mPa·s, the solid content is 38-42%, and the pH is 7-9; phthalocyanine sulfonic acid doped poly The volume ratio of aniline, water-based epoxy resin solution, leveling agent, defoamer, curing agent and thinner is 9~18:70~90:0.25~0.45:0.5~1.5:1~2:30~50.

[0022] Among them, the leveling agent is one of the BYK-3xx series produced by BYK Chemical Company, the curing agent is methyl etherified melamine formaldehyde resin, the defoaming agent is simethicone or BYK-020, BYK-028, and the diluent is One of ethylene glycol methyl ether, ethylene glycol ethyl ether or ethylene glycol butyl ether; t...

Embodiment l

[0026] 1) Synthesis of intrinsic polyaniline

[0027]Weigh 10ml of aniline monomer into a three-necked flask, then add 200ml of 1mol / l hydrochloric acid, add 50ml of xylene after stirring for 5 minutes, and form a uniform milky white emulsion after stirring for about 30 minutes; Ammonium sulfate aqueous solution 30ml, reacted at 15°C for 5 hours, filtered under reduced pressure after breaking the emulsification, and washed with distilled water until the filtrate was colorless. The filtered product was treated with 350ml of 8% ammonia water for 16 hours, the pH value was 8, filtered under reduced pressure, and the filter cake was vacuum-dried at 45°C to constant weight to obtain blue intrinsic state polyaniline.

[0028] 2) Synthesis of polyaniline doped with copper phthalocyanine sulfonic acid

[0029] Dissolve 10g of intrinsic polyaniline in 50ml of N,N-dimethylformamide (DMF), then add 130ml of an aqueous solution containing 20g of copper phthalocyanine disulfonic acid, hea...

Embodiment 2

[0033] 1) Synthesis of intrinsic polyaniline

[0034] Weigh 10ml of aniline monomer into a three-necked flask, then add 220ml of 1mol / l hydrochloric acid, add 55ml of xylene after stirring for 5 minutes, and form a uniform milky white emulsion after stirring for about 30 minutes; slowly add 13.5g of 30ml of ammonium persulfate aqueous solution, reacted at 14°C for 5 hours, filtered under reduced pressure after breaking the emulsification, and washed with distilled water until the filtrate was colorless. The filtered product was treated with 350ml of 8% ammonia water for 16 hours, the pH value was 8, filtered under reduced pressure, and the filter cake was vacuum-dried at 45°C to constant weight to obtain blue intrinsic state polyaniline.

[0035] 2) Synthesis of polyaniline doped with copper phthalocyanine sulfonic acid

[0036] Dissolve 10g of intrinsic polyaniline in 50ml of DMF, then add 150ml of an aqueous solution containing 25g of copper phthalocyanine disulfonic acid, ...

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PUM

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Abstract

The invention discloses phthalocyanine-based sulfonic acid-doped polyaniline anticorrosive paint which is prepared by the following method: (1), synthesizing eigenstate polyaniline; (2), synthesizing phthalocyanine-based sulfonic acid-doped polyaniline: taking and sufficiently dissolving the eigenstate polyaniline with N, N-dimethyl formamide, then, adding phthalocyanine-based sulfonic acid liquor, washing by using distilled water until filtrate is colorless after reacting for 10 hours-15 hours at 60 DEG C-70 DEG C, and vacuum-drying solids to obtain the phthalocyanine-based sulfonic acid-doped polyaniline; and (3), preparing polyaniline anticorrosive paint: under the room temperature, mixing the phthalocyanine-based sulfonic acid-doped polyaniline, aqueous epoxy resin liquor, a flatting agent and a de-foaming agent, dispersing for 10 minutes under 1500r / minute, filtering, and adding a curing agent and a diluent for sufficiently mixing to obtain the needed anticorrosive paint. The phthalocyanine-based sulfonic acid-doped polyaniline anticorrosive paint disclosed by the invention can effectively overcome a de-doping phenomenon, is simple to operate, good in adhesion force and excellent in corrosion resistance.

Description

technical field [0001] The invention relates to an anti-corrosion coating, in particular to a polyaniline anti-corrosion coating doped with phthalocyanine sulfonic acid, which can be used for anti-corrosion treatment of iron-based materials and belongs to the technical field of coatings. Background technique [0002] In 1985, DeBerry discovered that polyaniline has a protective effect on iron-based metals. After the metal surface is coated with polyaniline paint, it can effectively prevent air, water and salt from acting, and prevent metal from rusting and corroding. Moreover, this paint is non-toxic, It has the characteristics of low dosage, low density, good compatibility with organic resins, and convenient use. It has incomparable characteristics of ordinary coatings, such as anti-scratch, anti-pitting corrosion and prevention of marine organisms. These excellent characteristics have opened up polyaniline Anti-corrosion application of coatings under harsh conditions, such...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C09D163/00C09D179/02C09D5/08C08G73/02
Inventor 李明田杨瑞嵩王莹附青山崔学军金永中
Owner 四川宇涂科技有限公司