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A kind of preparation method of graphene oxide doped gel electrolyte

A technology of gel electrolyte and graphene, applied in hybrid capacitor electrolyte, capacitor electrolyte/absorbent, hybrid/electric double layer capacitor manufacturing, etc., to achieve good flexibility, avoid contact, and simple preparation method

Active Publication Date: 2020-11-27
HENAN NORMAL UNIV
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

Graphene oxide is added as an additive in the gel electrolyte, which can be formed in situ in the middle of the electrode. The porous dielectric layer similar to the diaphragm effectively avoids the deformation of the flexible capacitor device during assembly and use while ensuring the charge transfer of the electrolyte. The short circuit phenomenon caused by electrode contact, however, there is no relevant research report on this aspect

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0014] Step S1: using the Hummer method to prepare a graphene oxide aqueous solution, and then preparing a 2 mg / mL graphene oxide aqueous solution by dilution;

[0015] Step S2: Add 1 g of high polymer polyvinyl alcohol to 10 mL of the graphene oxide aqueous solution diluted in step S1, and stir and dissolve at 85° C. to form a uniform mixed solution;

[0016] Step S3: Add electrolyte phosphoric acid to the homogeneous mixed solution obtained in step S2, wherein the added mass of electrolyte phosphoric acid is 5% of the mass of the homogeneous mixed solution, and stir for 3 hours to obtain a dark brown uniform graphene oxide-doped gel electrolyte.

Embodiment 2

[0018] Step S1: using the Hummer method to prepare a graphene oxide aqueous solution, and then preparing a 1 mg / mL graphene oxide aqueous solution by dilution;

[0019] Step S2: Add 3 g of high polymer polyvinyl alcohol to 10 mL of the graphene oxide aqueous solution diluted in step S1, stir and dissolve at 90° C. to form a homogeneous mixed solution;

[0020] Step S3: Add concentrated sulfuric acid as electrolyte to the homogeneous mixed solution obtained in step S2, wherein the added mass of concentrated sulfuric acid as electrolyte is 10% of the mass of the homogeneous mixed solution, and stir for 4 hours to obtain a dark brown uniform graphene oxide-doped gel electrolyte.

Embodiment 3

[0022] Step S1: using the Hummer method to prepare a graphene oxide aqueous solution, and then preparing a 5 mg / mL graphene oxide aqueous solution by dilution;

[0023] Step S2: Add 2 g of high polymer polyacrylonitrile to 10 mL of the graphene oxide aqueous solution diluted in step S1, and stir and dissolve at 80° C. to form a uniform mixed solution;

[0024] Step S3: Add electrolyte potassium hydroxide to the homogeneous mixed solution obtained in step S2, wherein the added mass of electrolyte potassium hydroxide is 20% of the mass of the homogeneous mixed solution, and stir for 6 hours to obtain a dark brown uniform graphene oxide doped gel electrolyte.

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Abstract

The invention discloses a preparation method of a graphene oxide doped gel electrolyte. The method comprises the following steps: firstly, preparing graphene oxide by a Hummer method, and diluting toprepare a graphene oxide aqueous solution of a specific concentration; then adding high polymer polyvinyl alcohol or polyacrylonitrile; stirring under a heating condition to form a homogeneous mixed solution; then introducing concentrated sulfuric acid, phosphoric acid, potassium hydroxide and other electrolytes; and stirring to obtain a black and brown homogeneous graphene oxide doped gel electrolyte. The graphene oxide doped gel electrolyte prepared by the method has high structural toughness. Meanwhile, graphene oxide can be used as a porous dielectric layer to avoid contact between two poles of flexible devices, thereby reducing the phenomenon of electric leakage.

Description

technical field [0001] The invention belongs to the technical field of gel electrolyte preparation, and in particular relates to a preparation method of graphene oxide doped gel electrolyte. Background technique [0002] The rise of flexible electronic devices such as wearable energy devices has put forward higher requirements on the performance of electrolytes. The development of gel electrolytes with high flexibility, stretch-compressibility, high ionic conductivity, high power density, fast charge-discharge rate, and long cycle life has become an urgent need in this field. Gel electrolyte has the advantages of both liquid and solid electrolytes, making it an ideal electrolyte material. In the preparation of flexible electronic devices, it is necessary to avoid the contact of two electrodes and to reduce the distance between the two electrodes. However, there are still certain limitations in the current gel electrolyte, which hinders the further development of flexible el...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): H01G9/028H01G11/56H01G11/84
CPCH01G9/028H01G11/56H01G11/84Y02E60/13
Inventor 蒋凯邹肖肖武大鹏王红菊徐芳高志永
Owner HENAN NORMAL UNIV