Preparation method of hydroxy terminated polydimethylsiloxane with ring structure and application of method
The technology of hydroxypolysiloxane and hydroxypolydimethylsiloxane is applied in the field of preparation of hydroxyl base polymer with ring structure, which can solve the problems of poor physical and mechanical strength, crushing and cracking, high price, etc. The effect of improving mechanical properties, high elongation, and improving toughness
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[0029] The preparation method of the above-mentioned hydroxyl polysiloxane with ring structure comprises the following steps:
[0030] (1) Add 291 to 297 parts by weight of α, ω-dihydroxy polysiloxane and 0.3 to 1.5 parts by weight of platinum catalyst into a reactor with a constant temperature function, stir for 5 minutes, and set the temperature at 23±2°C Add 1.5-3 parts by weight of hydrogen-containing cyclic body dropwise, and stir for 5 minutes. Set the material temperature to 35°C;
[0031] (2) The temperature rises to 35±2°C, heat preservation reaction for 1.8 to 2 hours, add 0.01 to 0.05 parts by weight of 1-ethynyl-1-cyclohexanol, stir for 5 minutes, set the material temperature to 80°C; the stirring speed of the reaction 180-200 rpm;
[0032] (3) The temperature is raised to 80±2°C, and the low molecules are removed in vacuum for 1 hour, and the vacuum degree is -0.095MPa~-0.1MPa; the temperature is lowered, and the material is discharged to obtain a hydroxypolysil...
Embodiment 1
[0036] The raw materials used in this embodiment and the ratio of raw materials are as shown in Table 1:
[0037] Table 1 raw materials and proportioning:
[0038]
[0039] Using the ratio of raw materials in Table 1, the hydroxypolysiloxane with ring structure of the present invention is prepared through the following steps:
[0040] (1) Add the No. 1 and No. 2 materials into the reactor with constant temperature function, start stirring, and the rotation speed is 190 rpm. After 5 minutes, add No. 3 materials at 23±2°C, and set the material temperature to 35 ℃;
[0041] (2) The temperature rises to 35±2°C, heat preservation reaction for 1.8 hours, add the material in No. 4, and set the material temperature to 80°C;
[0042] (3) The temperature is raised to 80±2° C., and the low molecules are removed in vacuum for 1 hour; the temperature is lowered, and the material is discharged to obtain a hydroxy polysiloxane with a ring structure.
[0043] Add 1 part of tetraethoxysi...
Embodiment 2
[0045] The raw materials used in this embodiment and the ratio of raw materials are as shown in Table 2:
[0046] Table 2 raw materials and ratio
[0047]
[0048] Using the ratio of raw materials in Table 2, the hydroxypolysiloxane with ring structure of the present invention is prepared through the following steps:
[0049](1) Add the No. 1 and No. 2 materials into the reactor with constant temperature function, start stirring, and the rotation speed is 190 rpm. After 5 minutes, add No. 3 materials at 23±2°C, and set the material temperature to 35 ℃;
[0050] (2) The temperature rises to 35±2°C, heat preservation reaction for 1.8 hours, add the material in No. 4, and set the material temperature to 80°C;
[0051] (3) The temperature is raised to 80±2° C., and the low molecules are removed in vacuum for 1 hour; the temperature is lowered, and the material is discharged to obtain a hydroxy polysiloxane with a ring structure.
[0052] Add 1 part of tetraethoxysilane and 0...
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