A preparation method and application of a polyelectrolyte-coated nanofiltration composite membrane for treating electroplating wastewater
A polyelectrolyte and composite membrane technology, which is applied in the fields of metallurgical wastewater treatment, water/sewage treatment, chemical instruments and methods, etc., to achieve the effects of strong controllability, mild conditions and good pollution resistance
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[0071] The invention provides a preparation method of a nanofiltration composite membrane, comprising the following steps:
[0072] 1) After mixing the polyacrylonitrile and the first solvent, an intermediate film liquid is obtained, and then the intermediate film liquid is coated on the base film to obtain a carrier compounded with the intermediate film;
[0073] 2) After mixing polyethyleneimine, poly(2-hydroxylactone methacrylate), vinylpyrrolidone and the second solvent again, a cross-linked composite film liquid is obtained, and then the cross-linked composite film liquid is coated on the above steps On the intermediate film of the obtained carrier, after cross-linking by electron beam irradiation, solidification is performed to obtain a nanofiltration membrane carrier;
[0074] 3) The nanofiltration membrane carrier obtained in the above steps is immersed in a poly(4-styrenesulfonic acid) ammonium salt solution, taken out and then immersed in a polydimethyldiallyl ammoni...
Embodiment 1
[0125]To prepare an intermediate transition support layer, put 100 g of organic polyacrylonitrile into 900 g of N,N-dimethylformamide, stir to dissolve, and degassing to obtain an intermediate transition support layer membrane liquid. The interlayer film liquid is quantitatively coated on the non-woven fabric, and the solvent is evaporated to form the interlayer. 80 g of polyethyleneimine, 20 g of poly(4-styrenesulfonamide) ammonium salt and vinylpyrrolidone (1%) were dissolved in N,N-dimethylformamide to form a colloidal raw material, which was defoamed to obtain a composite layer film liquid. The composite layer film liquid was quantitatively coated on the intermediate layer, and the cross-linking dose was 60kGy using electron beam irradiation. The crosslinked membrane was immersed in pure water to solidify. The polyelectrolyte poly(4-styrenesulfonic acid) ammonium salt was dissolved in pure water to prepare a 0.2 wt% poly(4-styrenesulfonic acid) ammonium salt solution with...
Embodiment 2
[0131] To prepare an intermediate transition support layer, put 100 g of organic polyacrylonitrile into 900 g of N,N-dimethylformamide, stir to dissolve, and degassing to obtain an intermediate transition support layer membrane liquid. The interlayer film liquid is quantitatively coated on the non-woven fabric, and the solvent is evaporated to form the interlayer. 75 g of polyethyleneimine, 25 g of poly(4-styrenesulfonamide) ammonium salt and vinylpyrrolidone (1%) were dissolved in N,N-dimethylformamide to form a colloidal raw material, which was defoamed to obtain a composite layer film liquid. The composite layer film solution was quantitatively coated on the intermediate layer, and the cross-linking dose was 70kGy using electron beam irradiation. The crosslinked membrane was immersed in pure water to solidify. The polyelectrolyte poly(4-styrenesulfonic acid) ammonium salt was dissolved in pure water to prepare a 0.4 wt% poly(4-styrenesulfonic acid) ammonium salt solution w...
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