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Method for preparing resveratrol dimer

A technology of resveratrol and dimer, which is applied in the field of preparation of resveratrol dimer, can solve the problems of low specificity of oxidase, long reaction time, low conversion rate, etc., and achieve remarkable effect and synthetic The effect of shortening the time and improving the conversion efficiency

Inactive Publication Date: 2012-10-03
尉亚辉 +4
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

However, the main problems in the current enzymatic synthesis of resveratrol dimer are the low specificity of oxidases, long reaction time, and generally low conversion rate.

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0022] Step 1. Enzymatic synthesis of resveratrol dimer

[0023] Dissolve 1 kg of resveratrol in 8 L of acetone solution with a mass concentration of 40%, add 3 kg of porous sintered glass rings with immobilized laccase, react at 35°C for 2 hours, and release the reaction solution after the reaction; Add the acetone solution dissolved in resveratrol to the reactor (the solid phase of immobilized laccase is left) to continue the reaction. The immobilized laccase can be used repeatedly (as the enzyme activity decreases, the reaction time can be prolonged), and the reaction time is collected. solution until the activity of immobilized laccase was reduced by half.

[0024] Step 2. Isolation of resveratrol dimer

[0025] The collected reaction solution is precipitated with an organic solvent chloroform (methanol or ethanol can also be used) to precipitate proteins, after filtration, the liquid phase is concentrated to a quarter of the original volume, then ethyl acetate is added f...

example 2

[0027] Step 1. Enzymatic synthesis of resveratrol dimer

[0028] Dissolve 1kg of resveratrol in 9L of acetone solution with a mass concentration of 50%, add 3.5kg of porous sintered glass ring with immobilized laccase, react at 40°C for 3 hours, and release the reaction solution after the reaction is completed; Add resveratrol-dissolved acetone solution to the reactor (leaving the solid phase of immobilized laccase) to continue the reaction. The immobilized laccase can be used repeatedly (as the enzyme activity decreases, the reaction time can be prolonged), and the collected The reaction solution was changed until the enzyme activity of the immobilized laccase was reduced by half.

[0029] Step 2. Isolation of resveratrol dimer

[0030] The collected reaction liquid is precipitated with the organic solvent methanol (chloroform or ethanol can also be used) to precipitate the protein, after centrifugation, the liquid phase is concentrated to a quarter of the original volume, t...

example 3

[0032] Step 1. Enzymatic synthesis of resveratrol dimer

[0033]Dissolve 1kg of resveratrol in 9L of ethyl acetate solution with a mass concentration of 30%, add 4kg of porous sintered glass ring with immobilized laccase, react at 45°C for 3 hours, and release the reaction solution after the reaction; In the reactor (the solid phase of immobilized laccase is left), add ethyl acetate solution dissolved with resveratrol to continue the reaction, and the immobilized laccase can be used repeatedly (as the enzyme activity decreases, the reaction time can be prolonged) , collect the reaction solution, and replace it until the enzyme activity of the immobilized laccase is reduced by half.

[0034] Step 2. Isolation of resveratrol dimer

[0035] The collected reaction solution was precipitated with neutral salt sodium sulfate (ammonium sulfate or zinc sulfate can also be used) to precipitate protein, after centrifugation, the liquid phase was concentrated to one-fifth of the original...

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Abstract

The invention discloses a method for preparing a resveratrol dimer. The method is characterized by comprising the following steps of: dissolving resveratrol into acetone or ethyl acetate solution, adding immobilized laccase into the solution, reacting the solution for 1 to 5 hours at the temperature of between 35 and 45 DEG C, and then performing solid-liquid separation; and adding the solid phase containing the immobilized laccase into the reaction substrate for continuous reaction and reuse, depositing protein in the collected reaction solution by using an organic solvent or a neutral salt,concentrating the liquid phase after solid-liquid separation, adding ethyl acetate into the concentrate for extracting, concentrating the extract, and drying the concentrate to obtain the resveratroldimer. By adopting the immobilized laccase for the synthesis of the resveratrol dimer, the synthesis time can be greatly shortened (from 24 hours to 1-4 hours), the conversion efficiency is remarkably improved (from 18-21 percent to 35-38 percent), and the effect is remarkable.

Description

technical field [0001] The invention belongs to the technical field of biochemical synthesis, and in particular relates to a preparation method of resveratrol dimer. technical background [0002] Resveratrol (resveratrol) is a functional ingredient in grapes and wine, the molecular formula is C 14 h 12 o 3 , the relative molecular weight is 228.25, and the chemical name is 3,4′,5-trihydroxy-1,2-stilbene, which belongs to a class of compounds with a stilbene core—a non-flavonoid polyphenol compound with a stilbene structure. Resveratrol has a wide range of physiological activities, including anti-arteriosclerosis, anti-oxidation, anti-bacterial and anti-inflammatory, anti-tumor activity, cardiovascular protection, anti-AIDS activity, and immune regulation. Studies have shown that resveratrol has antagonistic effects on lung cancer, liver cancer, intestinal cancer, gastric cancer, breast cancer and leukemia. [0003] Resveratrol dimer is a kind of natural compound with com...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C12P7/22C12N11/08
Inventor 尉亚辉马丁郭斌程亚刚王芍
Owner 尉亚辉