Substrate and imageable element with hydrophilic interlayer
A technology for imaging elements and interlayers, applied in transportation and packaging, preparation of printing surfaces, and coating equipment for photographic plate-making processes, etc.
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Embodiment 1
[0213] Synthesis Example 1: Interlayer Compound A (IC-A):
[0214] Step 1: MEK (330.8 g, dried on molecular sieves), 100 g Jeffamine ED-2003 (0.10 equivalents, polyetherdiamine with a main polyethylene glycol backbone, MW=2000, purchased from Huntsman) and 5.06 g Triethylamine (0.05 eq.) was added to a four-necked 1000 ml flask equipped with a heating mantle, temperature controller, mechanical stirrer, condenser, pressure-balanced addition funnel, and nitrogen inlet. Then, 5.22 g (0.05 eq.) of methacryloyl chloride were added within 15 minutes at 25°C while keeping the reaction temperature below 35°C. After two hours the temperature was raised to 50°C and stirred for another hour. The reaction mixture was cooled to room temperature. Triethylamine hydrochloride (TEA: HCl salt) was removed by filtration. To the solution was added MEHQ (0.055 g). MEK was removed under vacuum (100 mm) and heat (45 °C). About 100 g of intermediate are obtained.
[0215] Step 2: The intermedia...
Embodiment 2
[0216] Synthesis Example 2: Interlayer Compound A1 (IC-A1):
[0217] Step 1: MEK (331.9 g, dried on molecular sieves), 90 g Jeffamine ED-900 (0.20 equivalents, polyetherdiamine with a main polyethylene glycol backbone, MW=2000, purchased from Huntsman) and 10.19 g Triethylamine (0.1 eq.) was added to a four-necked 1000 ml flask equipped with a heating mantle, temperature controller, mechanical stirrer, condenser, pressure-balanced addition funnel, and nitrogen inlet. Then, 10.45 g (0.1 eq.) of methacryloyl chloride were added within 15 minutes at 25°C while keeping the reaction temperature below 35°C. After two hours the temperature was raised to 50°C and stirred for another hour. The reaction mixture was cooled to room temperature. Triethylamine hydrochloride (TEA: HCl salt) was removed by filtration. To the solution was added MEHQ (0.055 g). MEK was removed under vacuum (100 mm) and heat (45 °C). About 90 g of intermediate are obtained.
[0218] Step 2: The intermediate ...
Embodiment 1
[0219] Comparative synthesis example 1: interlayer compound B (IC-B):
[0220] Step 1: MEK (330.8 g, dried on molecular sieves), 100.0 g polyethylene glycol (0.10 equivalent, MW=2000, purchased from Alfa Aesar) and 5.06 g triethylamine (0.05 equivalent) were added to a heating mantle , a temperature controller, a mechanical stirrer, a condenser, a pressure-balanced addition funnel, and a four-neck 1000 ml flask with nitrogen inlet. Then, 5.22 g (0.05 eq.) of methacryloyl chloride were added within 15 minutes at 25°C while keeping the reaction temperature below 35°C. After two hours the temperature was raised to 50°C and stirred for another hour. The reaction mixture was cooled to room temperature. Triethylamine hydrochloride (TEA: HCl salt) was removed by filtration. MEHQ (0.055 g) was added to the solution and MEK was removed under vacuum (100 mm) and heat (45 °C). About 90 g of intermediate are obtained.
[0221] Step 2: The intermediate from Step 1 (56.9 g, 0.0275 equi...
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