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A regeneration method for p507 extraction and separation of rare earth organic phase emulsion

A rare earth organic and organic phase technology, applied in the direction of improving process efficiency, can solve the problems of polluting the environment, wasting rare earth resources, etc., and achieve the effects of high recovery rate, simple and easy process, and low price

Inactive Publication Date: 2016-05-11
NANCHANG HANGKONG UNIVERSITY
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

Obviously, discarding the P507 organic phase emulsion in nature not only wastes precious rare earth resources and the more expensive extractant P507, but also pollutes the environment.

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0010] In a 1000L reaction pot, add 200kg of P507 organic phase emulsion and 150L of sodium hydroxide solution with a concentration of 6mol / L and a temperature of 95°C in sequence, stir and react for 8min, then stand still for 20min, and separate layers; the upper layer is a clear organic phase. phase, the middle layer is a transparent water phase, and the lower layer is a precipitate containing rare earth hydroxide. The water phase and sediment are released from the bottom of the reaction pot for recovery of rare earths. The upper organic phase is a regenerated P507 organic phase, which can be directly used for the extraction and separation of rare earths. The recovery rate of P507 organic phase was 99.5%.

[0011] The aqueous phase and precipitate that drained from the bottom of the reaction pot were filtered. The filtrate is sodium hydroxide solution, which is neutralized to pH ≈ 7 with hydrochloric acid solution and discharged. The precipitate is washed with deionized w...

Embodiment 2

[0013] In a 1000L reaction pot, add 200kg of P507 organic phase emulsion and 150L of sodium hydroxide solution with a concentration of 8mol / L and a temperature of 100°C in sequence, stir and react for 5min, then stand still for 30min, and separate layers; the upper layer is a clear organic phase. phase, the middle layer is a transparent water phase, and the lower layer is a precipitate containing rare earth hydroxide. The water phase and sediment are released from the bottom of the reaction pot for recovery of rare earths. The upper organic phase is a regenerated P507 organic phase, which can be directly used for the extraction and separation of rare earths. The recovery of the P507 organic phase was 100%.

[0014] The aqueous phase and precipitate that drained from the bottom of the reaction pot were filtered. The filtrate is sodium hydroxide solution, which is neutralized to pH ≈ 7 with hydrochloric acid solution and discharged. The precipitate is washed with deionized wa...

Embodiment 3

[0016] In a 1000L reaction pot, add 200kg of P507 organic phase emulsion and 150L of sodium hydroxide solution with a concentration of 4mol / L and a temperature of 90°C in sequence, stir and react for 10min, then stand still for 10min, and separate layers; the upper layer is a clear organic phase. phase, the middle layer is a transparent water phase, and the lower layer is a precipitate containing rare earth hydroxide. The water phase and sediment are released from the bottom of the reaction pot for recovery of rare earths. The upper organic phase is a regenerated P507 organic phase, which can be directly used for the extraction and separation of rare earths. The recovery of the P507 organic phase was 99%.

[0017] The aqueous phase and precipitate that drained from the bottom of the reaction pot were filtered. The filtrate is sodium hydroxide solution, which is neutralized to pH ≈ 7 with hydrochloric acid solution and discharged. The precipitate is washed with deionized wat...

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Abstract

A regeneration method for P507 extraction and separation of rare earth organic phase emulsion, the specific steps are: in a reaction pot, add P507 organic phase emulsion and 4? mol / L~8? mol / L sodium hydroxide solution at a temperature of 90°C to 100°C, stirred for 5? min~10? After 1 min, the layers were static; the upper layer was a clear organic phase, the middle layer was a transparent aqueous phase, and the lower layer was a precipitate containing rare earth hydroxide. Release the water phase and sediment from the bottom of the reaction pot, filter, wash, and dissolve with hydrochloric acid to recover the rare earths in them by oxalic acid precipitation, and the yield of rare earths is about 95%. The upper organic phase is a regenerated P507 organic phase, which can be directly used for the extraction and separation of rare earths. The recovery rate of the P507 organic phase of the present invention is high, reaching 99%-100%.

Description

technical field [0001] The invention relates to a regeneration method for P507 extraction and separation of rare earth organic phase emulsions, in particular to a regeneration method for treating P507 organic phase emulsions with hot sodium hydroxide solution, and belongs to the technical field of solvent extraction. Background technique [0002] P507 (2-ethylhexylphosphonic acid mono-2-ethylhexyl ester) is the most important extractant for industrial separation of mixed rare earth raw materials. In the process of P507 extraction and separation of rare earth elements, it is inevitable to encounter the problem of emulsification of the organic phase. In the rare earth extraction and separation production line, it is often necessary to remove the organic phase emulsion (also known as the emulsified three-phase). When the emulsification is serious, the production must be stopped to clean the tank. P507 organic phase emulsion usually contains rare earth, iron, silicon, calcium, ...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C22B3/38
CPCY02P10/20
Inventor 钟学明
Owner NANCHANG HANGKONG UNIVERSITY