Optical resin material, method for producing the optical resin material, optical resin member containing the material, and polarizing plate containing the same
A technology of optical resin and manufacturing method, applied in the direction of polarizing elements, etc., capable of solving problems such as insufficient offset
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Embodiment 1
[0110] (Design of monomer composition ratio)
[0111] In this example, choose figure 1 The 3 monomers shown in are PhMA (1st monomer), BzMA (2nd monomer) and EMI (3rd monomer), and design such that a copolymer is obtained by combining these monomers When , the characteristic birefringence and characteristic temperature coefficient of birefringence of the optical film made from the obtained copolymer are both zero. Specifically, the composition ratios of the above three types of monomers were determined by calculation using the following formulas (iv) to (vi) as described above.
[0112]
[0113]
[0114] 100=W 1 +W 2 +W 3 (vi)
[0115] Specifically, in this example, in order to design a copolymer capable of obtaining an optical thin film having both a characteristic birefringence and a characteristic birefringence temperature coefficient of zero, the above-mentioned simultaneous equations (iv) to (vi) are used to calculate Monomer formulations. When the intrinsi...
Embodiment 2
[0129] In the same manner as in Example 1 except that the mass ratio of the monomers of the copolymer was prepared as MMA / PhMA / BzMA=40 / 27 / 33, the film obtained from the copolymer was obtained at 25°C. The intrinsic birefringence and the intrinsic temperature coefficient of birefringence. As a result, the characteristic birefringence at 25°C is Δn 0 =-0.22×10 -3 , the temperature coefficient of characteristic birefringence is dΔn 0 / dT=0.38×10 -5 ℃ -1 , the thin film formed from the copolymer prepared in this example also showed little change in birefringence even if the temperature was increased, reducing the temperature dependence.
Embodiment 3
[0131] Except that the mass ratio of the monomers of the copolymer was prepared as a copolymer of a 3-component system of MMA / PhMA / EMI=29 / 54 / 17, the same operation was performed as in Example 1, and the monomer composition was designed so that the obtained unit Copolymers were synthesized by bulk composition. In addition, the intrinsic birefringence and the temperature coefficient of intrinsic birefringence at 25° C. were determined for the thin film obtained from the copolymer. Image 6 The results are shown in . As a result, the characteristic birefringence at 25°C is Δn 0 =-0.47×10 -3 , the temperature coefficient of characteristic birefringence is dΔn 0 / dT=-0.12×10 -5 ℃ -1 , the thin film formed from the copolymer prepared in this example also showed little change in birefringence even if the temperature was raised, reducing the temperature dependence.
[0132] (Measurement of temperature dependence of characteristic birefringence of polymers)
[0133] In the prese...
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