Liquid crystal aligning agent, liquid crystal alignment film and liquid crystal display element
A technology of liquid crystal alignment agent and liquid crystal alignment film, which is applied in liquid crystal materials, instruments, optics, etc. It can solve the problems of small anisotropy of polymer films, failure to obtain liquid crystal orientation, and image sticking, etc., and achieve good image sticking characteristics, suppression of bright spots, and high reliability
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[0144] The following examples are given to describe the present invention in more detail, but the present invention is not limited or interpreted by them.
[0145] The abbreviations and measurement methods of the compounds used in the following are as follows.
[0146] NMP: N-methyl-2-pyrrolidone
[0147] BCS: Butyl Cellosolve
[0148] DA-1: 1,2-bis(4-aminophenoxy)ethane
[0149] DA-2: 1,3-bis(4-aminophenoxy)propane
[0150] DA-3: p-phenylenediamine
[0151] DA-6: 4-(2-(Methylamino)ethyl)aniline
[0152]
[0153] [viscosity]
[0154] For the viscosity of polyamic acid ester and polyamic acid solution, using E-type viscometer TVE-22H (manufactured by Toki Sangyo Co., Ltd.), the sample volume is 1.1mL, and the cone rotor TE-1 (1 ° 34', R24) , Measured at a temperature of 25°C.
[0155] [molecular weight]
[0156] The molecular weight of the polyamic acid ester is measured using a GPC (normal temperature gel permeation chromatography) device, and the number average mol...
Synthetic example 1
[0182]Take DA-1 0.81g (3.30mmol), DA-20.57g (2.20mmol), DA-3 0.36g (3.30mmol), DA-4 0.88 g (2.20 mmol), NMP29.99g was added, and stirring and dissolution were carried out while feeding nitrogen gas. While stirring this diamine solution, 2.35 g (10.51 mmol) of 1,3-dimethyl-1,2,3,4-cyclobutanetetracarboxylic dianhydride was added so that the solid content concentration became 12 mass % to add NMP 6.40g and stir at room temperature for 24 hours to obtain a polyamic acid solution (A). The viscosity of this polyamic acid solution at a temperature of 25° C. was 316 mPa·s. In addition, the molecular weight of this polyamic acid was Mn=13230, Mw=29550.
Synthetic example 2
[0184] Take DA-1 0.54g (2.20mmol), DA-20.85g (3.30mmol), DA-3 0.36g (3.30mmol), DA-4 0.88 g (2.20 mmol), NMP30.17g was added, and stirring and dissolution were carried out while feeding nitrogen gas. While stirring this diamine solution, 2.35 g (10.51 mmol) of 1,3-dimethyl-1,2,3,4-cyclobutanetetracarboxylic dianhydride was added so that the solid content concentration became 12 mass % to add NMP 6.34g and stir at room temperature for 24 hours to obtain a polyamic acid solution (B). The viscosity of this polyamic acid solution at a temperature of 25° C. was 356 mPa·s. In addition, the molecular weight of this polyamic acid was Mn=14120, Mw=31210.
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