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Manufacturing method of polyacrylonitrile-based carbon fiber precursor

A technology of polyacrylonitrile-based carbon fiber and manufacturing method, which is applied in the field of preparing polyacrylonitrile-based carbon fiber precursors by wet spinning, and can solve the problems of poor mechanical properties of carbon fibers and easy generation of wool from precursors

Active Publication Date: 2021-06-22
CHINA PETROLEUM & CHEM CORP +1
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0008] Technical Problems Mainly Solved by the Invention In the prior art, polyacrylonitrile fibers are used as carbon fiber precursors in the process of preparing carbon fibers;

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0026] 1. Coagulation and drawing: Wet spinning is used to prepare primary fibers. The intrinsic viscosity of the stock solution used is 1.75dL / g, and the solid content of the spinning stock solution is 22%. , the spinneret hole diameter is 60 μm, the number of spinneret holes is 12000, the coagulation temperature is 25° C., the concentration is 50%, followed by two-stage coagulation and drawing, and the drawing ratio is 1.0 and 1.05 respectively to obtain coagulated fibers.

[0027] 2. Hot water drawing, water washing and oiling, low-temperature drying and drying densification: use 3-level hot water drawing, the drawing temperature is 90, 98, 99 ℃, and the drawing ratio is 1.8, 2.0, 2.4; water washing The temperature is 60°C, the draft ratio is 1.0; the oiling temperature is 35°C; the low temperature drying and densification temperature is 88°C.

[0028] 3. High-temperature drying and densification: the final drying and densification temperature is 135°C, the tension on each ...

Embodiment 2

[0035] 1. Coagulation and drafting: The primary fiber is prepared by wet spinning. The intrinsic viscosity of the stock solution used is 1.75dL / g, and the solid content of the spinning stock solution is 22%. The spinning stock solution is accurately metered by a metering pump and filtered again before spinning. The diameter of the spinneret is 60 μm, the number of spinneret holes is 12,000, the coagulation temperature is 25°C, and the concentration is 50%, followed by two-stage coagulation and drawing, and the drawing ratio is 1.0 and 1.05, respectively, to obtain coagulated fibers.

[0036] 2. Hot water drawing, water washing and oiling, low-temperature drying and drying densification: use 3-level hot water drawing, the drawing temperature is 90, 98, 99 ℃, and the drawing ratio is 1.8, 2.0, 2.4; water washing The temperature is 60°C, the draft ratio is 1.0; the oiling temperature is 35°C; the low temperature drying and densification temperature is 88°C.

[0037] 3. High-tempe...

Embodiment 3

[0044] 1. Coagulation and drafting: The primary fiber is prepared by wet spinning. The intrinsic viscosity of the stock solution used is 1.75dL / g, and the solid content of the spinning stock solution is 22%. The spinning stock solution is accurately metered by a metering pump and filtered again before spinning. The diameter of the spinneret is 60 μm, the number of spinneret holes is 12,000, the coagulation temperature is 25°C, and the concentration is 50%, followed by two-stage coagulation and drawing, and the drawing ratio is 1.0 and 1.05, respectively, to obtain coagulated fibers.

[0045] 2. Hot water drawing, water washing and oiling, low-temperature drying and drying densification: use 3-level hot water drawing, the drawing temperature is 90, 98, 99 ℃, and the drawing ratio is 1.8, 2.0, 2.4; water washing The temperature is 60°C, the draft ratio is 1.0; the oiling temperature is 35°C; the low temperature drying and densification temperature is 88°C.

[0046] 3. High-tempe...

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Abstract

The invention relates to a method for manufacturing polyacrylonitrile-based carbon fiber precursors, which mainly solves the problems in the prior art that the precursors are prone to wool and the mechanical properties of carbon fibers are poor. The present invention adopts a manufacturing method of polyacrylonitrile carbon fiber precursor, adopts wet spinning, and includes the step of drying and densification, wherein, the drying and densification includes at least two stages, and each strand in the last stage of drying and densification process The technical proposal that the tension the fiber bears is 1.5-3mN better solves this problem and can be used in the industrial production of polyacrylonitrile fibers.

Description

technical field [0001] The invention relates to a method for manufacturing polyacrylonitrile-based carbon fiber precursors, more specifically, the invention relates to a method for preparing polyacrylonitrile-based carbon fiber precursors by wet spinning. Background technique [0002] Carbon fiber is an inorganic fiber with a carbon content of 90% or more. It has a series of advantages such as light weight, high specific strength, high specific modulus, high temperature resistance, corrosion resistance, wear resistance, and fatigue resistance. Carbon fiber and various The composite material made by the composite process of the matrix has excellent performance, and has been widely used in the fields of automobile lightweight, wind power blades, sports and leisure products, etc. [0003] The precursors that can be used to prepare carbon fibers include three major raw material systems: polyacrylonitrile-based, viscose-based and pitch-based. Among them, polyacrylonitrile-based ...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): D01D5/06D01D5/12D01D10/06D01F6/18D01F6/38
CPCD01D5/06D01D5/12D01D10/06D01F6/18D01F6/38
Inventor 李磊沈志刚昌志龙赵微微
Owner CHINA PETROLEUM & CHEM CORP