Propylene-based polymer additives for improved tire tread performance
A technology of tire tread and diene terpolymer, applied in special tires, tire parts, transportation and packaging, etc.
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[0051] According to another embodiment of the present invention, the rubber composition comprises, for example, 30-100 phr, especially 50-100 phr (parts by weight / percent of total elastomer) of a high Tg elastomer as a compound of 0 to 70 phr, especially 0-50 phr A blend of low Tg elastomers; according to another example, it comprises 70-100 phr of low Tg elastomers exhibiting, for example, greater than 90%, or greater than 95% cis-1,4-linkage content levels (molar %) of polybutadiene (BR); according to another example, it contains all 100 phr of one or more SBRs prepared in solution.
[0052] According to another embodiment of the invention, the diene elastomer of the composition according to the invention comprises BR (as a low Tg elastomer) exhibiting a cis-1,4-structure level (mol %) greater than 90% Blends with one or more S-SBR or E-SBR as high Tg elastomer(s).
[0053] The compositions described herein may comprise a single diene elastomer or a mixture of several diene...
Embodiment
[0100] Seven propylene-ethylene-diene terpolymer (PEDM) additives (Table 1 ) were used in the tire tread formulations of the following examples.
[0101] Preparation of amorphous propylene-based copolymers (PEDM 1 to 7)
[0102] Catalyst system: The catalyst precursor is bis((4-triethylsilyl)phenyl)methylene(cyclopentadienyl)(2,7-di-tert-butyl-fluoren-9-yl)dimethyl Based hafnium. However, other metallocene precursors with good diene incorporation and MW capabilities can also be used.
[0103] The activator is dimethylanilinium tetrakis(pentafluorophenyl)borate, but dimethylanilinium tetrakis(heptafluoronaphthyl)borate and other non-coordinating anionic activators or MAO can also be used.
[0104] Polymerization experiments were performed in a Continuous Stirred Tank Reactor (CSTR) manufactured by Autoclave Engineers, Erie, PA. The reactor was designed to operate at a maximum pressure and temperature of 2000 bar (30 kpsi) and 225°C, respectively, but current experiments have...
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Abstract
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