2-furyl- and 2-thienyl-substituted di- and tetrahydropyrans for use as aroma chemicals
An O-C1-C4-, aromatic technology, applied in organic chemistry, food science, essential oils/fragrances, etc., can solve the problems that dihydropyran and tetrahydropyran have not been proposed as aroma chemicals
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[0342] Preparation Example
[0343] abbreviation:
[0344] DMAP: 4-(Dimethylamino)-pyridine
[0345] EA: ethyl acetate
[0346] RT: room temperature
[0347] THF: Tetrahydrofuran
[0348] MTBE: methyl-tert-butyl ether
[0349] analyze:
[0350] The purity of the product was determined on an area % basis by gas chromatography:
[0351] GC column: DB-WAX (30m (length), 0.25mm (ID), 0.25 micron (film));
[0352] Temperature program: 5 min at 50°C, 50°C to 230°C at 6°C / min, 10 min at 230°C. Injector temperature 200°C; detector temperature 230°C. Flow rate: 1.4ml / min
[0353] pass 13 The product was identified by C NMR.
[0354] 1a) Preparation of 2-(furan-2-yl)-4-methyl-tetrahydropyran-4-ol (R 1 =OH compound of formula (I.a)) and corresponding three elimination products with exocyclic or intracyclic double bonds (X=O and R 2 , R 3 or R 4 with R 1 Compounds of formula (I) that together represent a double bond)
[0355] To prenol (3-methylbut-3-en-1-ol) (40 g, 0...
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