Water Soluble Hydrophobically Associating Copolymer
A hydrophobic association and copolymer technology, applied in drilling compositions, chemical instruments and methods, etc., can solve the problems of high gel ratio, inability to completely eliminate, and polymer flooding damage.
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[0099] Preparation of Water-Soluble Hydrophobically Associating Copolymers
[0100] The copolymers of the invention can be prepared by free-radical polymerization of the monomers (a), (b) and optionally (d) by methods known in principle to those skilled in the art, for example by solution polymerization in aqueous phase or gel polymerization, but each possible polymerization variant must be carried out in the presence of at least one component (c).
[0101] The synthesis of the monomers (a) of the formula (I) used according to the invention is particularly preferably prepared by alkoxylation of alcohols (III) and optionally subsequent etherification according to the preparation methods described above.
[0102] In a preferred embodiment, the preparation takes place by gel polymerization in aqueous phase. For the gel polymerization, a mixture of monomers (a), (b) and optionally (d), initiators, surfactants (c) and further auxiliaries is first prepared together with water. Aci...
Embodiment
[0123] 1. Preparation method
[0124] 1.1 Preparation Example 1 (comparison): no surfactant is added during polymerization
[0125] First 242.5 g of a 50% Na AMPS solution (AMPS 2405, Lubrizol) were added to a 3 l vessel equipped with a stirrer and thermometer. 295.8 g of water were added with stirring. Then 1.2 g of Surfynol DF 58 and 0.4 g of Baysilone EN (Bayer) were added successively as antifoams. After adding 4.6 g of Pluriol A1190V+12PeO (a development product from BASF consisting of hydroxybutyl vinyl ether with 25 ethylene oxide units and 12 pentylene oxide units), 228.8 g of 50% concentration of acrylamide solution (Cytec). After adding 2.4 g of 5% Versenex solution to destabilize the acrylamide solution, use 20% NaOH solution and / or 20% H 2 SO 4 The pH of the solution was adjusted to 6.0. During inertization by purging with nitrogen for 30 minutes, the solution was cooled to about 20°C. The solution was then transferred to a plastic container with dimensions ...
preparation Embodiment 2-4
[0128] 1.2 Preparation Example 2-4 (the present invention): adding surfactant during gel polymerization
[0129] In addition to the monomer solution described in Comparative Example 2, prior to polymerization, Lutensol TO 15 (BASF, C13 oxo alcohol ethoxylate + 15 ethylene oxide units) was used as surfactant in the following amount Dissolved in monomer solution:
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