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A method for separating and refining non-basic nitrogen-containing compounds in petroleum fractions

A technology for petroleum fractions and nitrogen compounds, which is applied in the petroleum industry, multi-stage series refining process treatment, hydrocarbon oil treatment, etc., and can solve the problem of inability to separate non-basic nitrogen compounds in batches.

Active Publication Date: 2020-07-14
PETROCHINA CO LTD
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0004] The purpose of the present invention is to provide a method for separating and refining non-basic nitrogen-containing compounds in petroleum fractions, so as to solve the defect that non-basic nitrogen-containing compounds cannot be separated in batches in the prior art

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0034] The raw material oil is the extracted oil of transformer oil produced by the refinery, with a nitrogen content of 390 μg / g, a basic nitrogen content of 125 μg / g, and a sulfur content of 420 μg / g. Take 1000g of the raw oil sample, add 30g of phosphoric acid, stir at 50°C for 20 minutes, stop stirring, settle for 60 minutes, and divide into upper and lower layers. The upper layer oil is analyzed for its basic nitrogen content of 0.5 μg / g, indicating that the basic nitrogen content of the oil is 0.5 μg / g. Nitrogen has essentially been removed. Then pour out the upper layer of oil, be careful not to pour out the lower layer, then add 30g of tin tetrachloride, stir for 30 minutes, let stand for 200 minutes to separate the layers, use a separatory funnel to separate the lower layer, add petroleum ether at 60-90°C (analytical pure) 30ml, wash twice, separate the lower layer, then add petroleum ether 30ml, then add 15% NaOH solution 150ml, at this time the pH of the solution is...

Embodiment 2

[0036] Take 1000g of hydrogenated shale oil, its total nitrogen content is 12600mg L -1 , non-basic nitrogen content 7100mg·L -1 , dilute 4 times with petroleum ether, first add the WLDN denitrification agent developed by China University of Petroleum (East China) to remove the basic nitrogen compounds, the addition amount is 10% of the quality of hydrogenated shale oil, stir for 30 minutes, and the temperature 50°C, stop stirring and settling for 60 minutes after the reaction, divide into upper and lower layers, pour out the upper layer, and then add 150g of analytically pure SnCl to the separated upper layer oil 4, stirred and reacted for 30 minutes, the reaction temperature was controlled at 50°C, then stopped stirring, and settled and separated for 200 minutes. The solution was divided into upper and lower layers, and the lower layer was separated. Add 200ml of petroleum ether to the complex, wash, separate the petroleum ether, and repeat the washing once to obtain the wa...

Embodiment 3

[0042] Take vacuum distillate oil 1000g, its total nitrogen content is 875mg L -1 , non-basic nitrogen content 302mg·L -1 , sulfur content 580mg·L -1 , first add the WLDN denitrification agent developed by China University of Petroleum (East China) to remove the basic nitrogen compounds, the amount added is 2% of the quality of the vacuum distillate oil, and the reaction is stirred for 30 minutes at a temperature of 90 ° C. After the reaction, stop stirring and settling 120 minutes, divided into upper and lower layers, the basic nitrogen content in the upper layer oil is 1.6mg·L -1 , pour out the upper layer oil, then add 10g of analytically pure TiCl to the separated upper layer oil 4 , stirred and reacted for 60 minutes, the reaction temperature was controlled at 50°C, then stopped stirring, settled and separated for 200 minutes, the solution was divided into upper and lower layers, and the lower layer was separated. At this time, the non-basic nitrogen removal rate reache...

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Abstract

Provided is a method for separating and refining non-basic nitrogen-containing compounds in petroleum fractions. The method for separating and refining the non-basic nitrogen-containing compounds in the petroleum fractions includes the steps of: (1) adding denitrogenation agents to petroleum-free fractions containing no moisture, stirring and standing, and separating into an oil layer and a complex layer; (2) adding complexing agents to the oil layer obtained in the first step, stirring and standing, and separating into an oil layer and a complex layer; (3) adding low boiling hydrocarbons to the complex obtained in the second step, stirring and standing, separating into an oil layer and a complex layer, adding the low boiling hydrocarbons to the complex layer again and repeating the step;(4) adding low boiling point hydrocarbons to the complex layer finally obtained in step (3), adding alkali solution to neutralization so that the pH value is greater than 7, stirring and standing, andseparating into an oil layer and an aqueous layer; (5) washing the oil layer obtained in step (4) with deionized water, washing off remaining salt and alkali and keeping the oil layer; (6) separatingthe low boiling hydrocarbons from the washed oil layer obtained in step (5) to obtain residues, the non-basic nitrogen compounds.

Description

technical field [0001] The invention belongs to the field of refining petroleum and petroleum fractions, and relates to a method for separating and refining non-alkaline nitrogen-containing compounds in petroleum fractions. The International Patent Classification belongs to C10G. Background technique [0002] In the process of petroleum processing, various compounds in petroleum need to be separated to different degrees to determine the structure, properties and refining methods of this type of compound, and it becomes a difficult problem to separate and purify these compounds. Petroleum fractions are a mixture of organic compounds with different distillation ranges separated according to different boiling points in petroleum. The separation of various substances from these mixtures can be used to characterize, analyze properties, and predict processing methods for the fraction. Since oil contains thousands or even tens of thousands of organic compounds, it is very difficul...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C10G53/12
CPCC10G53/12C10G2300/202
Inventor 王会娟王延臻马书杰孙晨段红玲
Owner PETROCHINA CO LTD