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Polymeric dispersants for petroleum process streams

A technology of polymers and dispersions, which is applied in the petroleum industry, processing hydrocarbon oils, and devices for coating liquids on surfaces, etc., and can solve problems such as unsuitability of anhydride-functional polymers

Pending Publication Date: 2021-12-24
ECOLAB USA INC
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

Therefore, anhydride-functional polymers are not suitable for use in water-contaminated process streams

Method used

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Examples

Experimental program
Comparison scheme
Effect test

example 1

[0058] Copolymers of C24-C28 alpha-olefins with maleic anhydride (CAS No. 68459-79-0) were obtained according to the procedure outlined in Comer et al., US Patent No. 5,214,224. 50 g of polymer were then dispersed in 100 g of HAN (Heavy Aromatic Naphtha) and the dispersion was heated to 60-65°C with constant stirring. Then 20 g of oleylamine (20 g) was slowly added to the mixture over 30 minutes. The temperature of the reaction mixture was observed to rise to about 80°C. The mixture was stirred for an additional 2 hours while maintaining the temperature at 60-65°C. Anhydride peaks (1780 and 1711cm -1 ) disappearance and amide peak (1679cm -1 ) appears. No peak formation associated with imide groups was observed during the reaction.

[0059] When it was determined that the reaction was complete, another 100 g of HAN was added to the mixture, and the mixture was stirred for another 30 minutes. The mixture was then cooled to ambient temperature and filtered to remove traces...

example 2

[0061] The fouling of petroleum products in the presence of the polymer of Example 1 was determined by the following test method. Precipitation measured by this procedure predicts relative fouling behavior in petroleum process streams.

[0062] The equipment used in the experiment consisted of a 12.5 mL graduated conical centrifuge tube; a timer and a light box and / or a flashlight to facilitate observation of the sediment present in the dark petroleum liquid. In each test, centrifuge tubes were charged with a mixture of Crude A (from Tesoro Refinery, Anacortes, WA) or Crude B (Total Refinery, Port Arthur, TX) with 15 ppm of the antifouling polymer of Example 1; a mixture was formed by mixing the corresponding amount of the 26 wt% solids dispersion of Example 1 with the crude oil sample and then adding 10 mL of this mixture to a centrifuge tube. Allow the contents of the tube to stand at 20°C for 2 hours. After standing, measure the volume of the sediment at the bottom of the...

example 3

[0069] The pour point of petroleum products was determined using ASTM D-97 with HAN as solvent. A 15% by weight solids dispersion of Product C (alpha olefin / maleic anhydride copolymer) was found to have a pour point of -12°C. A 15% by weight dispersion of the polymer of Example 1 was found to have a pour point of -26°C in HAN. At -26°C, it was further observed that the dispersion of the polymer of Example 2 did not precipitate.

[0070] As can be appreciated from the foregoing, the polymer of Example 1 provides a concentrate with a pour point low enough to provide product pumpability and pourability in the field, even under the winter conditions commonly encountered. Additionally, the pumpable / pourable product comprising the polymer of Example 1 remained substantially single phase when subjected to temperatures as low as -26°C; ie, the dispersion was stable at this temperature.

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PUM

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Abstract

Disclosed herein are methods and compositions for reducing fouling by natural and synthetic foulants that tend to precipitate during petroleum collecting, processing, transporting, and storing. The method includes applying one or more antifouling polymers to a petroleum product to form a treated petroleum product, wherein fouling by the treated petroleum product is reduced and a stable dispersion is formed over a wide range of processing conditions. The one or more antifouling polymers include the polymerized residues of one or more alpha-olefins and maleic anhydride, further wherein the maleic anhydride residues are reacted with a primary amine. Concentrates of the antifouling polymers in solvents are stable and pourable at temperatures of 0 DEG C to -40 DEG C.

Description

[0001] This application is an international application with the application number PCT / US2017 / 064850 entering the Chinese national phase, the application number is "201780070340.3", the application date is December 06, 2017, and the invention name is "Polymer dispersant for petroleum process streams" "A divisional application of the invention patent application. technical field [0002] The present invention relates to polymeric dispersants for petroleum products and their use. Background technique [0003] Hydrocarbon processing plants, from refineries to petrochemical plants, suffer from fouling due to the deposition of hydrocarbon by-products deposited in heat exchangers, furnaces, water circulation loops, distillation columns, vessels, pipelines, overheads and other processing equipment. These by-products include various hydrocarbons that may be present in crude oil as well as by-products of hydrocarbon refining processes. Fouling of internal surfaces of processing equ...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): C08F210/14C08F222/06C08F8/32C10G75/04
CPCC08F8/32C10G75/04C08F210/14C08F222/06C08F2/005C10G2300/206C08F8/12C08F2810/30B05D5/08
Inventor K·索内A·赛义德
Owner ECOLAB USA INC