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Polyimide film, mfg method and application

A technology of polyimide film and polyamic acid, applied in chemical instruments and methods, coatings, layered products, etc., can solve difficult and unclear problems

Inactive Publication Date: 2004-06-09
KANEKA CORP
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

However, more specific parameters such as (1) coefficient of linear expansion, (2) coefficient of hygroscopic expansion, and (3) modulus of elasticity are used when evaluating the above-mentioned physical properties, and it is not clear that all of these parameters will be in the optimum range. , and it is very difficult to adjust all the values ​​of these parameters (1) to (3) to the optimal range

Method used

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Examples

Experimental program
Comparison scheme
Effect test

preparation example Construction

[0092] The organic solvent used in the preparation of the polyamic acid solution, that is, the polymerization solvent used in the polymerization of the polyamic acid, is not particularly limited as long as it dissolves the polyamic acid. As a specific example, amide-based solvents, namely N-N-dimethylformamide, N-N-dimethylacetamide, N-methyl-2-pyrrolidone, etc. can be mentioned. Even among these, N-N- Dimethylformamide, N-N-dimethylacetamide. These organic solvents are usually used alone, but they can also be used in combination of two or more as needed.

[0093] In addition, the composition of the polyamic acid solution is not particularly limited, but the polyamic acid is preferably dissolved in an organic solvent in an amount of 5 to 35% by weight, most preferably 10 to 30% by weight. In such a range, a suitable molecular weight and solution viscosity can be obtained.

[0094] Fillers may be added to the above-mentioned polyimide film for the purpose of improving various...

Embodiment 1

[0143] In 407.5 g of N,N-dimethylformamide (DMF), 21.98 g of 4,4'-hydroxydiphenylamine (ODA) and 7.91 g of p-phenylenediamine (PDA) were dissolved, and the solution was kept at 0°C. To this solution, 29.47 g of 3,3'-4,4'-benzophenonetetracarboxylic dianhydride (BTDA) was gradually added, stirred for 1 hour, and BTDA was completely dissolved. Slowly add 25.15g p-phenylene bis(trimellitic monoester anhydride) (TMHQ) in this solution, after stirring for 1 hour, add 7.98g pyromellitic dianhydride (PMDA) again, stir for 1 hour hours, a polyamic acid solution having a solution viscosity of 3000 poise at 23° C. and a solid content concentration of 18.5% by weight was obtained. Table 1 shows the mol % of the monomer components added at this time. In Table 1 and Table 3 described later, the monomer compositions are described from the top to the bottom in the order of adding the monomers.

[0144] A curing agent consisting of 11.4 g of acetic anhydride, 4.8 g of isoquinoline, and 33.8...

Embodiment 2

[0147] 17.90 g of ODA and 9.67 g of PDA were dissolved in 407.5 g of DMF, keeping the solution at 0°C. 28.81 g of BTDA was slowly added to this solution, and stirred for 1 hour to completely dissolve BTDA. After slowly adding 24.59 g of TMHQ to this solution and stirring for 1 hour, 11.52 g of BTDA was added and stirred for 1 hour to obtain a polyamic acid solution having a solution viscosity of 2800 poise at 23° C. and a solid content concentration of 18.5% by weight. Table 1 shows the mol % of the monomer components added at this time. In addition, in Table 1, the mol% of BTDA is 50 and 20, and represents the amount of BPDA added first and BPDA added later.

[0148] Except having used this polyamic-acid solution, it produced similarly to Example 1, and obtained the polyimide film and TAB tape of thickness 50 micrometers. Table 2 shows the properties of the polyimide film and the TAB tape.

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PUM

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Abstract

This invention relates to a kind of polyimide film, which comprises 3,3',4,4'-benzophenonetetracarboxylic dianhydride and can satisfy physical properties such as mean linear expansion coefficient between 100 and 200 DEG C being above 18 ppm / DEG C and below 28 ppm / DEG C, elastic modulus being greater than 4.5 GPa, and coefficient of expansion caused by moisture absorption being below 13 ppm. Due to fulfilling all of the three physical property requirements, the polyimide film which prevents warping or curling from occurring in the TAB tape and flexile printed circuit board processing steps can be realized.

Description

technical field [0001] The present invention relates to a representative example of a polyimide film widely used as an insulating material, a method for producing the polyimide film, and an application thereof as the weight and size of various electronic devices become lighter and smaller. An example of the production method and utilization of a polyimide film used as a base film processed into a flexible printed wiring board (Flexible printed wiring board) or a TAB (Tape Automated Boding) tape. Background technique [0002] In the past, the flexible printed circuit board (abbreviated as FPC) effectively utilized its flexibility and was mainly folded and used in the small space inside the camera. However, in recent years, FPCs have been widely used in drive units such as floppy disk drives (FDD), hard disk drives (HDD), copiers, printers, etc., and therefore the sliding flexibility of FPCs is required to be further improved. [0003] FPC uses a resin film as a base, which i...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): C08G73/10B29C41/12B32B15/08C08J5/18C08L79/08H05K1/03
CPCB29C41/12B32B15/088C08G73/10C08G73/1007C08J5/18H05K1/03
Inventor 金城永泰松胁崇晃赤堀廉一
Owner KANEKA CORP