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Nano-filtration membrane for separating organic compounds and salts, and preparation method thereof

A technology of nanofiltration membrane and organic matter, which is applied in the field of nanofiltration membrane for separating organic matter and salt and its preparation, can solve the problems of poor pollution resistance, low separation efficiency, etc. Effect

Active Publication Date: 2013-08-07
艾德迈(北京)科技有限公司
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

However, when the existing nanofiltration membrane is applied to the above separation system, there are still problems such as low separation efficiency and poor pollution resistance.

Method used

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Examples

Experimental program
Comparison scheme
Effect test

preparation example Construction

[0015] The steps of the preparation method of the nanofiltration membrane for separating organic matter and salt are as follows:

[0016] 1) Add 3 to 6 parts by mass of monomers containing zwitterionic groups and 1 part by mass of hydroxyalkyl acrylate monomers into water to prepare an aqueous solution with a mass percent concentration of 10 to 30wt%, blow nitrogen into it, and add mass A water-soluble oxidation-reduction initiator with a percentage concentration of 1 to 3 wt%, at 30 to 45 o Solution polymerization is carried out at C, the polymerization time is 1 to 5 hours, and after several times of centrifugation and water washing, a binary copolymer containing zwitterions is obtained, which is vacuum-dried and used for later use;

[0017] 2) Add 1 to 2.5 parts by mass of the above-mentioned binary copolymer containing zwitterions and 0.1 to 0.45 parts by mass of polyaldehyde to disperse in water, then add inorganic acid to adjust the pH value of the solution to 1.8 to 3.8...

Embodiment 1

[0022] 6 parts by mass of 3-[N,N-dimethyl-[2-(2-methylprop-2-enoyloxy) ethyl] ammonium] propane-1-sulfonic acid inner salt and 1 part by mass The hydroxyethyl acrylate monomer is added into water to prepare an aqueous solution with a mass percentage concentration of 10wt%, and nitrogen gas is passed through, and an oxidation-reduction initiator K with a mass percentage concentration of 1% is added 2 S 2 o 8 and NaHSO 3 (1:1), at 45 o Solution polymerization is carried out under C, and the polymerization time is 1 hour. After several times of centrifugation and water washing, a binary copolymer containing zwitterions is obtained, which is dried in vacuo for subsequent use; 1 mass part of binary copolymers containing zwitterions and 0.1 The glutaraldehyde of mass part adds water and disperses, then adds sulfuric acid and adjusts solution pH value to be 1.8, at 20 o Stir at a temperature of C for 20 minutes to obtain a milky white dispersion; o Under the temperature of C and...

Embodiment 2

[0024] 3 parts by mass of 3-[N,N-dimethyl-[2-(2-methylprop-2-enoyloxy) ethyl] ammonium] propane-1-sulfonic acid inner salt and 1 part by mass The hydroxyethyl acrylate monomer is added into water to form an aqueous solution with a mass percentage concentration of 30wt%, and nitrogen gas is passed through, and an oxidation-reduction initiator K with a mass percentage concentration of 3% is added 2 S 2 o 8 and NaHSO 3 (1:1), at 30o Solution polymerization was carried out under C, and the polymerization time was 5 hours. After several times of centrifugation and water washing, a binary copolymer containing zwitterions was obtained, which was dried in vacuo for subsequent use; 2.5 parts by mass of binary copolymers containing zwitterions and 0.45 The glutaraldehyde of mass part adds water to disperse, then adds sulfuric acid and adjusts solution pH value to be 3.8, at 30 o Stir at a temperature of C for 40 minutes to obtain a milky white dispersion; o Under the temperature of ...

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Abstract

The present invention discloses a nano-filtration membrane for separating organic compounds and salts, and a preparation method thereof. The nano-filtration membrane of the present invention comprises a porous polysulfone support layer and an amphion-containing copolymer adopted a functional layer. The preparation process comprises: carrying out a solution polymerization reaction to obtain the amphion-containing copolymer; preparing the amphion-containing copolymer and a cross-linking agent into an aqueous dispersion with a certain concentration; carrying out impregnating for the surface of the porous polysulfone support membrane by the aqueous dispersion; carrying out curing cross-linking to obtain the composite membrane. According to the present invention, the composite nano-filtration membrane has water flux of 20-30 L.m<-2>.h<-1> under operation pressure of 0.6 MPa; the nano-filtration membrane provides the retention rate more than 90% for the organic compound molecules with the molecular weight more than 800, and provides the retention rate less than 20% for the inorganic salt molecules; the preparation method of the present invention is simple, the reaction conditions are mild, and the production cost is low; with the nano-filtration membrane, the good separation performance is provided for the organic compounds and the inorganic salts, and the good industrial application prospect is provided.

Description

technical field [0001] The invention belongs to the field of nanofiltration membrane separation, in particular to a nanofiltration membrane for separating organic matter and salt and a preparation method thereof. Background technique [0002] Nanofiltration is a new pressure-driven membrane separation process developed in the late 1980s. The pore size range of nanofiltration membrane is about 1-5nm, which is a kind of separation membrane between reverse osmosis membrane and ultrafiltration membrane. Nanofiltration membranes are generally charged membranes, which can separate inorganic salts of different valence states and various organic substances through the dual effects of pore size sieving and electrostatic repulsion. Nanofiltration separation technology has been widely used in water softening, wastewater treatment, biopharmaceutical, petrochemical and other fields in recent years because of its advantages such as no phase change, no heating, no damage to the characteri...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): B01D71/68B01D71/06B01D69/10B01D69/12B01D67/00
Inventor 安全福计艳丽高从堦
Owner 艾德迈(北京)科技有限公司