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Inorganic nanometer-sized mesoporous antibacterial agent and preparation method thereof

A technology of inorganic nanometer and antibacterial agent, applied in the fields of botanical equipment and methods, biocides, disinfectants, etc., can solve the problem that the loading percentage of antibacterial substances is not particularly high, and achieve the effect of simple preparation process

Inactive Publication Date: 2012-05-30
ZHEJIANG SCI-TECH UNIV
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

But the loading percentage of antimicrobial substances is not particularly high

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0020] 1) Dissolve 5.00 g of P123 in 161.7 mL of deionized water, add hydrochloric acid to make the pH of the solution lower than 2, stir until it settles, add 12.50 g of tetraethyl orthosilicate, 0.73 g of triethyl phosphate and 8.50 g of Ca (NO 3 ) 2 4H 2 O, stirred at 70°C for 72 hours, dried, and calcined at 550°C for 6 hours to obtain an inorganic nano-mesoporous material. (Silicon dioxide: calcium oxide: phosphorus pentoxide is 60:36:4).

[0021] 2) Amino-modify the prepared nano-mesoporous material, amino-modification process route: disperse each gram of inorganic mesoporous material in 100ml deionized water toluene and 1ml KH550, reflux in 80°C water bath reflux device for 5 hours, Then use a suction filter bottle with a pore size of 0.22 micron microporous membrane to filter and clean, and place the cleaned bioactive glass in a vacuum oven at 130°C for 12 hours to obtain an amino-modified inorganic nanometer mesoporous material;

[0022] 3) Take 5 g of the amino-m...

Embodiment 2

[0025] 1) Dissolve 4.50 grams of F104 in 445.5 mL of deionized water, add sulfuric acid to make the pH of the solution lower than 2, stir until it settles, add 19.23 g of butyl orthosilicate, 2.81 g of trimethyl phosphate and 4.44 g of CaCl2, Stir at 100° C. for 36 hours, and after drying, calcinate at 650° C. for 6 hours to obtain an inorganic nano-mesoporous material. (silicon dioxide: calcium oxide: phosphorus pentoxide is 60:40:10).

[0026] 2) Carry out mercapto-grafting of the prepared nano-mesoporous material; process route of mercapto-modification: disperse each gram of inorganic mesoporous material in 10ml of 0.1mol / L cysteamine hydrochloride solution, and treat at 80°C 24 hours, centrifugal filtration, repeated washing with deionized water, and then drying at 60°C to obtain mercapto-modified inorganic nano-mesoporous materials;

[0027] 3) Take 5g of the mercapto-modified inorganic nano-mesoporous material obtained above and add it to 50ml deionized water, drop in 1...

Embodiment 3

[0030] 1) Dissolve 3 grams of F65 in 597mL of deionized water, add nitric acid to make the pH of the solution lower than 2, stir until it settles, add 13.70g of methyl orthosilicate and 1.58g of calcium acetate, and stir at 120°C for 1 day , after drying, calcined at 700° C. for 6 hours to obtain inorganic nano-mesoporous materials. (Silicon dioxide: calcium oxide is 90:10).

[0031] 2) Amino-modify the prepared nano-mesoporous material, amino-modification process route: disperse each gram of inorganic mesoporous material in 100ml deionized water toluene and 1ml KH550, reflux in 80°C water bath reflux device for 5 hours, Then use a suction filter bottle with a pore size of 0.22 micron microporous membrane to filter and clean, and place the cleaned bioactive glass in a vacuum oven at 130°C for 12 hours to obtain an amino-modified inorganic nanometer mesoporous material;

[0032] 3) Take 5 g of the above-mentioned amino-modified inorganic nano-mesoporous material and add it to ...

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PUM

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Abstract

The invention discloses an inorganic nanometer-sized mesoporous antibacterial agent and a preparation method thereof. The preparation method comprises: agitating a polyethylene glycol-polypropylene glycol-polyethylene glycol block copolymer, deionized water and an acid together, adding a silicon source, a calcium source and a phosphorus source to obtain a sol-gel liquid, drying and sintering to obtain an inorganic nanometer-sized mesoporous material, carrying out amino or mercapto graft modification to obtain a modified inorganic nanometer-sized mesoporous material, adding the modified inorganic nanometer-sized mesoporous material to the deionized water or ethanol, dripping a silver nitrate solution, loading sliver and putting to a formaldehyde deionized water solution so that the sliver ions are reduced to a simple substance sliver, filtering, washing and drying. The loaded sliver is converted into the simple substance sliver through a strong reduction system, due to the graft modification, more sliver ions can be loaded in the mesoporous material, the content of the sliver is up to 25% of the weight of the whole antibacterial agent at most and higher than any one sliver-loading antibacterial product at present, and the product can be widely used in the fields of textiles, cleaning solvents, cosmetics, water treatment, plastics and the like.

Description

technical field [0001] The invention relates to an inorganic nanometer antibacterial agent material and a preparation method, in particular to an inorganic nanometer mesoporous silver-loaded antibacterial agent and a preparation method. technical background [0002] In modern life, there are a large number of viruses, bacteria, fungi and other microorganisms in the environment, which not only pollute the environment, but also directly lead to the occurrence and infection of many diseases, posing a great threat to human health. In recent years, due to the impact of "SARS", "bird flu" and "H1N1 influenza", people's awareness of hygiene has been continuously enhanced, and the demand for antibacterial materials and their products has greatly increased. [0003] There are currently three main categories of antimicrobial agents: organic, natural, and inorganic. Organic antibacterial agents have disadvantages such as poor weather resistance, short antibacterial effect, and large e...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): A01N59/16A01N25/08A01P1/00
Inventor 冯新星陈建勇张华鹏朱海霖周岚
Owner ZHEJIANG SCI-TECH UNIV