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Method for preparing uniform polymer beads

A polymer particle, uniform technology, applied in peptide preparation methods, biochemical equipment and methods, chemical instruments and methods, etc., can solve problems such as poor stabilizer, suspension failure, bead fusion, etc.

Inactive Publication Date: 2011-08-03
ROHM & HAAS CO
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0005] The anionic surfactants used in these processes are often good emulsifiers but generally poor stabilizers when used to polymerize uniform polymer beads
Instability often causes beads to fuse, potentially failing suspension

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0061] Example 1 : Preparation of 58 micron GMA / GlyDMA porous particles in a 20 liter reactor

[0062] Into a 10-liter stainless steel vessel equipped with an overhead stirrer was added 3,213 grams of deionized water. The reactor was heated to 80° C., and 32.5 grams of Gohsenol GR-14R PVOH produced by Nippon GOHSEI, Japan, were slowly added within 30 minutes. The PVOH solution was stirred at a temperature of 80°C for 1 hour and then cooled to 30°C.

[0063] In another 30-liter vessel, 9,707 grams of deionized water was added, and the vessel was heated to 55° C. with stirring at 100 rpm. Slowly add 48.8 grams of Methocel, manufactured by The Dow Chemical Company, Philadelphia, PA, to the container over a period of 1 minute. TM K100, heat to 80°C and keep for 15 minutes. The vessel was cooled to 25°C.

[0064] In another 10-liter container, add 2,019 grams of the prepared PVOH solution, 924.6 grams of GMA, 616.4 grams of GlyDMA, 2,457.7 grams of DEP, 753.3 grams of MIBC a...

Embodiment 2

[0066] Example 2 Preparation of 60 µm GMA / GlyDMA Porous Particles

[0067] Add 321 grams of deionized water to a 600 mL beaker equipped with a magnetic stirrer. The beaker was heated to 80°C and 3.25 grams of Gohsenol GR-14R PVOH was slowly added over a period of 10 minutes. The PVOH solution was stirred at a temperature of 80°C for 1 hour and then cooled to 30°C.

[0068] In another beaker, add 970 grams of deionized water, then heat the beaker to 80°C and stir with a magnetic stirrer. To this beaker was slowly added 4.88 grams of Methocel K100 over a period of 10 minutes. The Methocel was stirred at a temperature of 80°C for 1 hour and then cooled to 25°C.

[0069] 201.9 grams of the prepared PVOH solution, 92.46 grams of GMA, 61.64 grams of EGDMA, 245.7 grams of DEP, 753.3 grams of MIBC (4-methyl-2-pentanol) and 2.13 grams of tert-butyl peroctoate were added to a 1-liter beaker. The mixture was stirred at 400 rpm for 10 minutes.

[0070] In a 2-liter glass reactor e...

Embodiment 3

[0071] Example 3 Preparation of 30 µm GMA / EDGMA Porous Particles

[0072] Add 300 g of deionized water to a 600 mL beaker equipped with a magnetic stirrer. The beaker was heated to 80°C and 3 grams of Gohsenol GR-14R PVOH was slowly added over a period of 10 minutes. The PVOH solution was stirred at a temperature of 80°C for 1 hour and then cooled to 30°C.

[0073] In another beaker, 75 grams of deionized water was added, then the beaker was heated to 80°C and stirred using a magnetic stirrer. To this beaker was slowly added 6.25 grams of Methocel K100 over a period of 10 minutes. The Methocel was stirred at a temperature of 80°C for 1 hour and then cooled to 25°C.

[0074] 228.2 g of the prepared PVOH solution, 74.1 g of GMA, 49.4 g of EGDMA, 229.5 g of DEP and 1.8 g of tert-butyl peroctoate were added to a 1-liter beaker, and the mixture was stirred at 400 rpm for 10 minutes.

[0075] In a 1 liter glass reactor equipped with an overhead stirrer and condenser, 198.0 gr...

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Abstract

The invention discloses a method for preparing substantially uniform polymer particles in an aqueous dispersoid. The method comprises forming a monomer emulsion with an emulsifying agent, at least one monomer molecule, and an initiator; adding at least one stabilizing agent and a plurality of oligomeric droplets into the monomer emulsion; and polymerizing the at least one monomer molecule to form an aqueous dispersoid of polymer particles.

Description

technical field [0001] The present invention relates to a process for preparing polymer beads. More specifically, the present invention relates to methods for preparing substantially uniform polymer beads. Background technique [0002] To prepare polymer beads using the seed expansion technique, the monomer phase can be emulsified using surfactants such as sodium lauryl sulfate and Triton TM X-450. A method for preparing polymer beads is disclosed in U.S. Patent Publication No. 2007 / 0066761, in which seed particles are mixed with monomers, initiators, chain transfer agents, and surfactants to form The swellable particles are then mixed with monomers and initiators to polymerize. [0003] US Patent No. 5,147,937 describes another method of preparing particulate beads which involves gradually mixing a monomer mixture with emulsion polymerized polymer particles in the presence of a dispersion stabilizer and an oil soluble initiator. [0004] Another method of making polyme...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): C08F220/32C08F212/08C08F220/18C08F222/14C08F2/24C08F8/00C08J9/28C12N9/00C07K1/14
CPCC08F2/44C08F2/24
Inventor M·迪兹W·扎布罗德斯基J·J·迈克纳
Owner ROHM & HAAS CO