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Method for activating catalyst for chlorine production and method for producing chlorine

A technology of activation method and manufacturing method, which is applied in the direction of catalyst regeneration/reactivation, chemical instruments and methods, physical/chemical process catalysts, etc., can solve the problems of catalyst activity reduction, etc., and achieve the effect of reducing catalyst cost and good catalyst activity

Inactive Publication Date: 2012-04-11
SUMITOMO CHEM CO LTD
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

However, when the catalyst for chlorine production used in the above-mentioned reaction is subjected to a heat load under stable or unstable conditions, for example, the catalytic activity may decrease.

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0049] 5 g of the degraded catalyst obtained in Reference Example 1 and 45 g of a 36% hydrochloric acid aqueous solution (manufactured by Wako Pure Chemical Industries, Ltd.) were put into a container, mixed, and allowed to stand at 25° C. for 24 hours to bring them into contact. Subsequently, the supernatant was removed by decantation, and the resulting solid was washed three times with 150 g of ion-exchanged water, and then dried at 60° C. to reach a constant weight (more than 2 hours), to obtain the activated lysate activated by the activation method of the present invention. Catalyst (activated catalyst). In addition, when the pH of the 36% hydrochloric acid aqueous solution used here was measured, it was -2.0.

[0050] Next, the catalyst activity when the reaction of oxidizing hydrogen chloride with oxygen was performed using the obtained activated catalyst was evaluated by the following method. The results are shown in Table 1.

[0051]

[0052] 1 g of the obtained c...

Embodiment 2

[0056] Instead of the 36% aqueous hydrochloric acid solution used in Example 1, 45 g of a 20% aqueous hydrochloric acid solution (prepared by diluting 25 g of a 36% aqueous hydrochloric acid solution (manufactured by Wako Pure Chemical Industries, Ltd.) with 20 g of ion-exchanged water) was used. Except that, in the same manner as in Example 1, a catalyst (activated catalyst) activated by the activation method of the present invention was obtained. In addition, the pH of the 20% hydrochloric acid aqueous solution used here was measured and found to be -1.7.

[0057] Next, the catalyst activity when the reaction of oxidizing hydrogen chloride with oxygen was performed using the obtained activated catalyst was evaluated by the same method as in Example 1. The results are shown in Table 1.

Embodiment 3

[0059] Instead of the 36% aqueous hydrochloric acid solution used in Example 1, 45 g of a 2.5% aqueous hydrochloric acid solution (prepared by diluting 3.125 g of a 36% aqueous hydrochloric acid solution (manufactured by Wako Pure Chemical Industries, Ltd.) with 41.875 g of ion-exchanged water) was used, except Otherwise, in the same manner as in Example 1, a catalyst (activated catalyst) activated by the activation method of the present invention was obtained. In addition, the pH of the 2.5% hydrochloric acid aqueous solution used here was measured and found to be 0.2.

[0060] The catalyst activity when the reaction of oxidizing hydrogen chloride with oxygen was performed using the obtained activated catalyst was evaluated by the same method as in Example 1. The results are shown in Table 1.

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PUM

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Abstract

Disclosed is a method for activating a catalyst for chlorine production used in a reaction for oxidizing hydrogen chloride with oxygen, which comprises a step wherein a catalyst for chlorine production having decreased activity is brought into contact with an acidic liquid. Also disclosed is a method for producing chlorine, wherein chlorine is produced by oxidizing hydrogen chloride with oxygen in the presence of a catalyst for chlorine production that is activated by the above-described method. The acidic liquid used in the method preferably has a pH of not more than 5, and is preferably an aqueous solution in which an inorganic acid is dissolved. In addition, the catalyst for chlorine production preferably contains ruthenium oxide.

Description

technical field [0001] The present invention relates to a method for activating a catalyst for chlorine production whose activity has decreased, and a method for producing chlorine using the catalyst for chlorine production activated by the method. Background technique [0002] Chlorine is useful as a raw material for vinyl chloride, phosgene, and the like, and has conventionally been produced by a reaction in which hydrogen chloride is oxidized with oxygen in the presence of a catalyst for chlorine production. However, when the catalyst for chlorine production used in the above reaction is subjected to a heat load under stable or unstable conditions, for example, the catalytic activity may decrease. [0003] Therefore, as a method of activating a catalyst for chlorine production whose activity has decreased (hereinafter sometimes referred to as "deteriorated catalyst"), a method of contacting a degraded catalyst with a gas containing substantially only oxygen and / or an iner...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): B01J23/96B01J38/60C01B7/04
CPCC01B7/04B01J23/96B01J23/462B01J38/60Y02P20/584
Inventor 内田洋平关航平
Owner SUMITOMO CHEM CO LTD