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A kind of composite metal oxide catalyst for preparing biodiesel

A composite metal, biodiesel technology, applied in metal/metal oxide/metal hydroxide catalysts, physical/chemical process catalysts, biofuels, etc., can solve the problems of large amount of catalyst and difficult separation of products, etc. Short, good reuse effect, and the effect of many catalytic active sites

Inactive Publication Date: 2016-04-27
SHANGHAI UNIV
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

However, if the amount of catalyst is too large, it will cause saponification reaction, and the product is not easy to separate

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0014] Weigh 25mmol (2.78g) of CaCl respectively 2 , 50 mmol (11.95 g) MgCl 2 ·7H 2 O and 25 mmol (6.0375 g) of AlCl 3 ·6H 2 O, dissolved in 50 mL without CO 2 Prepare a mixed salt solution in water, and at the same time weigh 187.50mmol (7.5g) NaOH and dissolve it in 100mL tap water to prepare a mixed alkali solution. Under the action of magnetic stirring, slowly add the mixed salt solution to the NaOH solution at a rate of 15mL per minute , sealed at room temperature and magnetically stirred for 6 hours, and after standing for 4 hours, a white precipitate was formed. After taking it out, the mixed solution and the precipitate were filtered with suction, and washed repeatedly with distilled water for 2 to 3 times. The solid sample was dried at 105°C to obtain the ternary species Hydrotalcite, its structural formula is: Ca 0.24 Mg 0.46 al 0.30 (OH) 2 (Cl) 0.30 0.3H 2 O The obtained ternary hydrotalcites were calcined at 700°C for 3 hours to obtain composite metal oxi...

Embodiment 2

[0017] Weigh 25mmol (5.90g) of Ca(NO 3 ) 2 4H 2 O, 50mmol (12.82g) of Mg(NO 3 ) 2 ·6H 2 O and 25mmol (9.38g) of Al(NO 33 9H 2 O, dissolved in 50mL deionized water to prepare a mixed salt solution, at the same time weigh 187.50mmol (7.5g) NaOH and dissolve it in 100mL tap water to prepare a mixed alkali solution, and slowly add the mixed salt solution to the NaOH solution under the action of magnetic stirring , the drop rate is 15mL per minute, sealed with magnetic stirring at room temperature for 6 hours, and after standing for 4 hours, a white precipitate is formed. After taking it out, the mixed solution and precipitate are filtered with suction, washed 2~3 times with distilled water, and the solid sample is kept at 105 ° C. Drying at the bottom to obtain ternary hydrotalcite, its structural formula is: Ca 0.24 Mg 0.48 al 0.28 (OH) 2 (NO 3 ) 0.28 0.4H 2 O, the obtained ternary hydrotalcite was calcined at 700°C for 3 hours to obtain the final calcium-based solid...

Embodiment 3

[0020] Weigh 25mmol (4.30g) of CaSO 4 2H 2 O, 50 mmol (12.32 g) of MgSO 47H2O and 25mmol (16.66g) of Al 2 (SO 4 ) 3 18H 2 O, dissolved in 50mL deionized water to prepare a mixed salt solution, and at the same time weigh 187.50mmol (7.5g) NaOH and dissolve it in 100mL tap water to prepare a mixed alkali solution; under the action of magnetic stirring, slowly add the mixed salt solution to the NaOH solution , the dropping rate is controlled at 15mL per minute, sealed with magnetic stirring at room temperature for 6 hours, and a white precipitate is formed after standing for 4 hours. After taking it out, the mixed solution and precipitate are filtered with suction, and washed repeatedly with distilled water for 2 to 3 times. The solid sample is kept at 105°C Drying at the bottom to obtain the ternary hydrotalcite, the structural formula is: Ca 0.24 Mg 0.44 al 0.32 (OH) 2 (SO 4 ) 0.16 0.6H 2 O, the obtained ternary hydrotalcite was calcined at 700°C for 3 hours to obta...

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PUM

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Abstract

The invention relates to a composite metal oxide catalyst for preparing biodiesel. The catalyst belongs to the field of solid alkalis, and is a composite metal oxide obtained by carrying out high-temperature calcination on a precursor calcium-base hydrotalcite. The biodiesel prepared by the composite metal oxide provided by the invention is prepared by dropwisely adding vegetable fat, animal fat or waste edible fat into methanol or ethanol in a mol ratio of 1:(3-18) at the certain rate to carry out ester exchange reaction, wherein the conversion rate reaches 98% or so. The prepared biodiesel conforms to the BD100 main performance indexes. The composite metal oxide for preparing biodiesel has the advantages of cheap and accessible catalyst, favorable crystallinity, large specific area, high stability, multiple catalytic activity sites and favorable reutilization effect, and has favorable environment-friendly characteristic; the biodiesel preparation process has the advantages of low catalyst consumption, mild reaction conditions, short reaction time, high product yield and simple after-treatment.

Description

technical field [0001] The invention relates to a composite metal oxide catalyst, in particular to a solid base catalyst used for preparing biodiesel, and belongs to the field of catalysts and new energy sources. Background technique [0002] Biodiesel is a mixture of fatty acid esters prepared by transesterification of small molecule alcohols (methanol or ethanol) with animal and vegetable oils. Compared with petrochemical resources, biodiesel produced by this method has many advantages: such as cetane number, high lubrication , excellent performance, biodegradable, non-toxic, and less harmful emissions in the exhaust gas, so it is favored by countries all over the world. The catalysts used in the production of biodiesel can be divided into three categories: homogeneous catalysts, heterogeneous catalysts, and enzyme catalysts. Among them, the homogeneous catalyst has been industrially produced, but the problems such as difficult regeneration and large amount of three waste...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): B01J23/02C11C3/10
CPCY02E50/10
Inventor 陆永生张在屋杨芹伟马娟娟钱光人
Owner SHANGHAI UNIV