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A preparation method of tubular manganese dioxide array composite electrode material

A manganese dioxide and composite electrode technology, applied in the field of composite materials, can solve the problems of lack of application and low utilization rate of manganese dioxide, and achieve the effects of good stability, short preparation period and large specific surface area.

Active Publication Date: 2018-12-14
WUHAN INSTITUTE OF TECHNOLOGY
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

However, the pseudocapacitance provided by manganese dioxide mainly occurs in the region near the electrode surface and other regions are not used.
This leads to a lower utilization rate of manganese dioxide

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0020] The clean nickel sheet is evenly coated with the cellulose acetate film casting solution containing carbon nanotubes, so that a microfiltration membrane with uniform pore size can be formed on the nickel sheet. The casting solution is the membrane material - the polymer compound is dissolved in a good solvent, and the porogen is added to form a microfiltration membrane polymer solution under certain conditions.

[0021] Put the nickel sheet after the above treatment into 0.1mol / L potassium permanganate solution, make the potassium permanganate solution permeate and adsorb on the inner wall of the microfiltration membrane, and then treat it at a high temperature of 200°C for 30 minutes to obtain an oriented tubular array Structure of manganese dioxide.

[0022] Treat the above-mentioned nickel sheet in a nitrogen atmosphere at a high temperature of 400°C for 50 minutes, and let it cool down to room temperature naturally after the high-temperature treatment to obtain a ma...

Embodiment 2

[0025] The clean titanium sheet is evenly coated with the polysulfone casting solution containing carbon nanotubes, so that a polysulfone microfiltration membrane with uniform pore size can be formed on the titanium sheet.

[0026] Put the above treated titanium sheet into 1mol / L potassium permanganate solution, make the potassium permanganate solution infiltrate and adsorb on the inner wall of the polysulfone microfiltration membrane, and then treat it at 250°C for 90 minutes to obtain oriented tubular Array structure of manganese dioxide.

[0027] Put the treated titanium sheet in an argon atmosphere at a high temperature of 500°C for 60 minutes, and let it cool down to room temperature naturally after the high temperature treatment to obtain a manganese dioxide / carbon nanotube / carbon composite electrode material.

[0028] Add 1M Na to the electrode material prepared by the above steps 2 SO 4 The electrochemical performance test was carried out in the solution. The measure...

Embodiment 3

[0030] The clean nickel sheet is evenly coated with the cellulose acetate film casting solution containing carbon nanotubes, so that a cellulose acetate microfiltration membrane with uniform pore size can be formed on the nickel sheet.

[0031] Put the above treated nickel sheet into 1mol / L manganese chloride solution, make the manganese chloride solution infiltrate and adsorb on the inner wall of the cellulose acetate microfiltration membrane, and then treat it at 300°C for 100 minutes to obtain an oriented tubular array structure of manganese dioxide

[0032] Treat the above-mentioned nickel sheet in a nitrogen atmosphere at a high temperature of 600°C for 30 minutes, and let it cool down to room temperature naturally after the high-temperature treatment to obtain a manganese dioxide / carbon nanotube / carbon composite electrode material.

[0033] Add 1M Na to the electrode material prepared by the above steps 2 SO 4 The electrochemical performance test was carried out in the...

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Abstract

The invention discloses a preparation method of tubular manganese dioxide array composite electrode material. The preparation method comprises the following steps that a casting film solution containing carbon nanotubes is uniformly coated on a clean metal sheet so that an organic microfiltration film with uniform apertures is formed on the metal sheet; the metal sheet is immersed in a 0.1-6mol / L manganese containing solution and then processed for 30-200min under high temperature of 200-400 DEG C so that manganese dioxide with a directional tubular array structure is formed on the metal sheet; and the metal sheet is arranged in the atmosphere of inert gas to be processed for 30-180min under high temperature of 400-1000 DEG C so that the manganese dioxide / carbon nanotube / carbon composite electrode material is formed on the metal sheet. Manganese dioxide has the directional tubular array structure, and the carbon nanotubes / carbon fills around manganese dioxide. Conductivity of the composite electrode material can be enhanced and energy density and power density of a supercapacitor can also be enhanced by the structure.

Description

technical field [0001] The invention belongs to the technical field of composite materials, and relates to a method for preparing a tubular array type composite electrode material Background technique [0002] Supercapacitors, also known as electrochemical capacitors, are also called energy storage capacitors or Faraday capacitors. A supercapacitor is a new type of energy storage device between batteries and traditional physical capacitors. Supercapacitors have the characteristics of high energy density, long cycle life, high current charge and discharge, fast charge and discharge, etc., so they have broad application prospects and have received extensive research and attention in recent years. The electrode is the core component of the supercapacitor, which directly affects the performance of the supercapacitor. The function of the electrode is to store and release charge, which is the key to determine the charge storage capacity of the capacitor. Therefore, the electrode...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): H01G11/86H01G11/24H01G11/30H01G11/46H01G11/36H01G11/38
CPCY02E60/13
Inventor 王升高刘星星崔丽佳陈睿皮晓强张维
Owner WUHAN INSTITUTE OF TECHNOLOGY