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A preparation method of epoxy soybean oil modified low shrinkage sheet molding compound

A technology of epoxidized soybean oil and sheet molding compound, which is applied in the field of polymer material preparation, can solve the problems of micro-cracks, bubbles, pinholes, high curing shrinkage, low shrinkage and the like on the surface of sheet molding compound. Achieve low curing shrinkage, high surface smoothness, good fluidity and filling performance

Active Publication Date: 2019-02-12
宁波昌亚新材料科技股份有限公司
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0004] The technical problem to be solved by the present invention: Aiming at the problem that the sheet molding compound produced with unsaturated polyester resin as the base material has a high curing shrinkage rate, which makes the surface of the sheet molding compound prone to micro-cracks, air bubbles, pinholes, etc., provide A modified epoxy soybean modified alcohol was prepared by mixing with phthalic anhydride, maleic anhydride and other substances, then heated in a water bath, then added epoxy soybean modified alcohol, and heated in an oil bath to obtain a modified low shrinkage unsaturated polyester , and finally grind it with polystyrene low-shrinkage agent and conductive mica powder, then coat it on polyethylene film, roll it up, mature it, and cold press it to prepare sheet molding compound.

Method used

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Examples

Experimental program
Comparison scheme
Effect test

example 1

[0019] First, weigh 85 parts of epoxidized soybean oil, 2 parts of p-chlorophenylboronic acid, 3 parts of polyvinyl alcohol and 10 parts of propylene glycol in a three-necked flask, stir and mix them, and place them in a constant temperature water bath at 0.3 MPa and 85°C. Heat for 2 hours; after the water bath heating is completed, stop heating and let it stand to cool to 30°C, then add dropwise a 15% sodium hydroxide solution to adjust its pH to 8.5, stir and mix, and place it in a water bath to heat at 60°C 30min, then stop heating and vacuum distillation, collect the residual liquid remaining after vacuum distillation and suction filtration, collect the filtrate to prepare epoxy soybean modified alcohol, for subsequent use; then measure 30 Parts of phthalic anhydride, 10 parts of maleic anhydride, 15 parts of dicyclopentadiene, 10 parts of epoxy soybean modified alcohol prepared above and 35 parts of deionized water are placed in a four-necked flask, and then under nitrogen...

example 2

[0021] First, weigh 75 parts of epoxidized soybean oil, 3 parts of p-chlorophenylboronic acid, 7 parts of polyvinyl alcohol and 15 parts of propylene glycol in a three-necked flask, stir and mix them, and place them in a constant temperature water bath at 0.2MPa and 70°C. Heat for 1 hour; after the water bath heating is completed, stop heating and let it stand to cool to 20°C, then add dropwise a 15% sodium hydroxide solution to adjust its pH to 8.5, stir and mix, and place it in a water bath to heat at 45°C 15min, then stop heating and vacuum distillation, collect the residual liquid remaining after vacuum distillation and suction filtration, collect the filtrate to prepare epoxy soybean modified alcohol, for subsequent use; then measure 10 parts by weight respectively Parts of phthalic anhydride, 15 parts of maleic anhydride, 20 parts of dicyclopentadiene, 15 parts of epoxy soybean modified alcohol prepared above and 40 parts of deionized water are placed in a four-necked fla...

example 3

[0023]First, weigh 80 parts of epoxidized soybean oil, 2 parts of p-chlorophenylboronic acid, 7 parts of polyvinyl alcohol and 11 parts of propylene glycol in a three-necked flask, stir and mix them, and place them in a constant temperature water bath at 0.3 MPa and 80 °C. Heat for 2 hours; after the water bath heating is completed, stop heating and let it stand to cool to 25°C, then add dropwise a 15% sodium hydroxide solution, adjust its pH to 8.5, stir and mix, and place it in a water bath at 50°C for heating 20min, then stop heating and vacuum distillation, collect the residual liquid remaining after vacuum distillation and suction filtration, collect the filtrate to prepare epoxy soybean modified alcohol, for subsequent use; then measure 20 Parts of phthalic anhydride, 10 parts of maleic anhydride, 20 parts of dicyclopentadiene, 10 parts of epoxy soybean modified alcohol prepared above and 40 parts of deionized water are placed in a four-necked flask, and then under nitrog...

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Abstract

The invention relates to a preparation method for an epoxidized soybean oil-modified flaky molding compound with low shrinkage, which belongs to the technical field of preparation of high polymer materials. The preparation method comprises the following steps: mixing prepared epoxidized soybean oil-modified alcohol with substances like phthalic anhydride and maleic anhydride and carrying out heating in a water bath; then adding epoxidized soybean oil-modified alcohol and carrying out heating in an oil bath so as to obtain modified unsaturated polyester with low shrinkage; and grinding the modified unsaturated polyester, a polystyrene low-shrinkage agent and conductive mica powder, coating a polyethylene film with the obtained powder and then successively carrying out rolling, reeling, curing, cold pressing and molding so as to obtain the flaky molding compound. The flaky molding compound prepared in the invention has low cure shrinkage, lower than 0.01%, and good fluidity and filling properties.

Description

technical field [0001] The invention relates to a preparation method of epoxy soybean oil modified low-shrinkage sheet molding compound, which belongs to the technical field of polymer material preparation. Background technique [0002] Sheet molding compound is a raw material for molding made of unsaturated polyester resin, low shrinkage agent, glass fiber, filler and various additives. It has superior electrical properties and corrosion resistance, especially mechanical properties comparable to some metal materials, so it is widely used in transportation vehicles, construction, electrical and electronic industries. At the same time, due to the advantages of low raw material cost, high productivity, stable and reliable product quality, low environmental pollution, and high degree of automation, sheet molding compound (SMC) has been widely used in the production of FRP composite products and other fields. [0003] The matrix material used in sheet molding compound (SMC) is ...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C08L67/08C08L25/06C08L29/04C08K13/02C08K3/22C08K3/34C08G63/91C08G63/49
CPCC08G63/48C08G63/91C08K2201/001C08K2201/014C08L67/08C08L2205/03C08L25/06C08L29/04C08K13/02C08K2003/2296C08K3/34
Inventor 陈毅忠薛培龙高玉刚
Owner 宁波昌亚新材料科技股份有限公司