Polyfunctional polymerizable compound and colored composition
A compound and general formula technology, applied in the field of coloring compositions and multifunctional polymeric compounds, can solve the problems of hue change, brightness decrease, low heat resistance of dyes, etc., and achieve the effect of high dissolution resistance
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Synthetic example 1
[0757] Synthesis of Synthesis Example 1 Intermediate (Compound 2)
[0758] In a round-bottomed flask equipped with a stirring device, 2.0 g (3.9 mmol) of rhodamine B (compound 1: manufactured by Wako Pure Chemical Industries, Ltd.) and 2.7 g (3.9 mmol) of tetrakis(pentafluorophenyl)boron were added. (IV) Lithium salt (LiFABA) (manufactured by Tosoh Finechem Co., Ltd.) and 30 ml of methylene chloride were reacted at 25° C. for 1 hour. The reaction liquid was diluted with dichloromethane, and washed with water. The solvent was distilled off from the reaction solution by concentrating under reduced pressure to obtain 4.1 g of a purple solid carboxylate (Compound 2) having tetrakis(pentafluorophenyl)boron(IV) anion (100% yield).
[0759]
Embodiment 1
[0760] Synthesis of embodiment 1 polyfunctional polymerizable dye (compound 4)
[0761] In a round-bottomed flask equipped with a stirring device, 4.4 g (3.9 mmol) of the intermediate (compound 2) obtained in Synthesis Example 1 and 30 ml of dichloromethane were added for dissolution, and 2.4 g (4.7 mmol) of pentaerythritol tris Acrylate {compound 3: trade name Light Acrylate (Light Acrylate) PE-3A (compound 3 content: 60.0%), manufactured by Kyoeisha Chemical Co., Ltd.}, 0.1 g (1.2 mmol) of 4-dimethyl Aminopyridine (4-dimethylaminopyridine, DMAP) (manufactured by Wako Pure Chemical Industries, Ltd.) and 1.3 g (6.7 mmol) of 1-ethyl-3-(3-dimethylaminopropyl) carbodiimide salt Acid salt (1-ethyl-3-(3-dimethylaminopropyl)carbodiimide, WSC) (manufactured by Toyobo Co., Ltd.), was reacted at 25°C for 3 hours. The reaction solution was washed with water, and the solvent was distilled off from the reaction solution by concentration under reduced pressure to obtain a purple solid. T...
Embodiment 2
[0763] The synthesis of embodiment 2 polyfunctional polymeric dyes (compound 6)
[0764] In a round-bottomed flask equipped with a stirring device, 8.8 g (7.9 mmol) of the intermediate (compound 2) obtained in Synthesis Example 1 and 60 ml of methylene chloride were added and dissolved, and 12.4 g (9.4 mmol) of dipentaerythritol was added Pentaacrylate {compound 5: the trade name is NK ester A-9550 (the content of compound 5 is 40.0%), manufactured by Shin-Nakamura Chemical Co., Ltd.}, 0.3 g (2.4 mmol) of DMAP (Wako Pure Chemical Industries Co., Ltd. ) and 2.6 g (13.4 mmol) of WSC (manufactured by Toyobo Co., Ltd.), were reacted at 25° C. for 3 hours. The reaction solution was washed with water, and the solvent was distilled off from the reaction solution by concentration under reduced pressure to obtain a purple solid. Add 1300ml of methanol to the solid for dissolution, slowly dropwise add 300ml of water for crystallization, and then concentrate under reduced pressure to re...
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