Vinyl ethers and processes for their preparation
A vinyl ether, alkenyl technology, used in cationic curing agent or 1-component or 2-component system, used in the field of preparation of UV adhesives
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Embodiment 1
[0235]
[0236] Reaction scheme 1
[0237] Vinylation at room temperature
[0238] A round bottom flask (1000 mL) was charged with (0.5 mol%; 638.4 mg) Pd(OOCCF) 3 ) and (0.5 mol %; 300 mg) 2,2'-bipyridine. Subsequently, ethyl vinyl ether (15 equiv; 415 mL) and (1.6 mL; 3 mol%) NEt were added 3 . The mixture was stirred for 10 minutes. After this time (40 g; 0.384 moles) 1,4-pentanediol was added. During the course of the reaction (48 hours), the flask was sealed and stirred at room temperature. The catalyst was filtered off by using a pleated filter, followed by distillation of excess ethyl vinyl ether from the resulting filtrate on a rotary evaporator (40° C., 700 mbar→300 mbar). The crude mixture was then distilled under vacuum in order to obtain the first fraction (P-2-divin only) at 45°C and 0.5 mbar and at 60°C and 0.1 mbar Second fraction (mixture of P-1-prim. and P-1-secondary (P-1-sek.)).
[0239] Conversion of 1,4-pentanediol: 96%
[0240] Yield of P-2-d...
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