Organic-inorganic complex, and forming composition thereof
a technology of organic-inorganic complexes and complexes, applied in the direction of coatings, etc., can solve the problems of poor adhesion, easy cracking of films, poor adhesion,
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example 1
1) Preparation of Polysiloxane
[0140]17.00 g of methyltrimethoxysilane (Shin-Etsu Chemical Co., Ltd., KBM-13) was charged in a 140 mL mayonnaise bottle. 3.02 g of diisopropoxybisacetylacetonatotitanium (Nippon Soda Co., Ltd., T-50, the amount of the solid content in terms of TiO2: 16.5 wt %) was added so as to be 5 mol % in terms of TiO2 with respect to methyltrimethoxysilane. 19.91 g of MIBK was charged and stirred for 15 minutes (rate of stirring of 100 rpm).
[0141]4.50 g of distilled water was charged so as to be 2 times the mole of methyltrimethoxysilane, and a hydrolysis reaction was performed (2 hours, rate of stirring of 100 rpm). The liquid temperature rose to 40° C. at this time. After completion of the reaction, the reaction liquid was left for 30 minutes until the liquid temperature became 25° C.
2) Preparation of Organic-Inorganic Complex
[0142]In order to be dipentaerythritolhexaacrylate (Daicel-Cytec Company Ltd., DPHA, SP value of 10.40) / polysiloxane=90 wt % / 10 wt %, 17.3...
example 2
1) Preparation of Polysiloxane
[0144]17.00 g of methyltrimethoxysilane (Shin-Etsu Chemical Co., Ltd., KBM-13) was charged in a 140 mL mayonnaise bottle. 3.02 g of diisopropoxybisacetylacetonatotitanium (Nippon Soda Co., Ltd., T-50, the amount of the solid content in terms of TiO2: 16.5 wt %) was added so as to be 5 mol % in terms of TiO2 with respect to methyltrimethoxysilane. 19.91 g of MIBK was charged and stirred for 15 minutes (rate of stirring of 100 rpm).
[0145]4.50 g of distilled water was charged so as to be 2 times the mole of methyltrimethoxysilane, and a hydrolysis reaction was performed (2 hours, rate of stirring of 100 rpm). The liquid temperature rose to 40° C. at this time. After completion of the reaction, the reaction liquid was left for 30 minutes until the liquid temperature became 25° C.
2) Preparation of Organic-Inorganic Complex
[0146]In order to be VYLON 600 (registered trademark, TOYOBO CO., LTD, amorphous polyester resin) / polysiloxane=wt % / 10 wt %, 17.37 g of VY...
example 3
1) Preparation of Polysiloxane
[0148]17.00 g of methyltrimethoxysilane (Shin-Etsu Chemical Co., Ltd., KBM-13) was charged in a 140 mL mayonnaise bottle. 3.02 g of diisopropoxybisacetylacetonatotitanium (Nippon Soda Co., Ltd., T-50, the amount of the solid content in terms of TiO2: 16.5 wt %) was added so as to be 5 mol % in terms of TiO2 with respect to methyltrimethoxysilane. 19.91 g of MIBK was charged and stirred for 15 minutes (rate of stirring of 100 rpm).
[0149]4.50 g of distilled water was charged so as to be 2 times the mole of methyltrimethoxysilane, and a hydrolysis reaction was performed (2 hours, rate of stirring of 100 rpm). The liquid temperature rose to 40° C. at this time. After completion of the reaction, the reaction liquid was left for 30 minutes until the liquid temperature became 25° C. After that, water and an alcohol were removed by dehydrating distillation.
2) Preparation of Organic-Inorganic Complex
[0150]In order to be T-150 (Nippon Soda Co., Ltd., NISSO TITA B...
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