Diene polymer and process for producing the same
A technology of polymers and compounds, applied in the field of diene polymers
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[0169] The invention is explained with reference to the following examples, which do not limit the scope of the invention.
reference example 1
[0171] The preparation of 4-(tert-butyldimethylsilyloxy group)-1,6-heptadiene represented by formula (3)
[0172] Into a 100 ml two-necked flask was charged 6.5 g of imidazole manufactured by Wako Pure Chemical Industries, and then 50 ml of anhydrous N,N-dimethylformamide manufactured by the above company and 5.78 ml of 1 , 6-heptadien-4-ol. The resulting mixture was cooled to 0 °C. To this mixture was added 6.5 g of tert-butyldimethylsilyl chloride manufactured by Tokyo Chemical Industry Co., Ltd., and the resulting mixture was stirred at room temperature for 12 hours. An excess of water was then added thereto to terminate the reaction. The product contained in the reaction mixture was extracted with hexane, and the obtained organic extract was dried over anhydrous sodium sulfate manufactured by Nacalai Tesque Inc. Company. The dried hexane solution was vacuum distilled to obtain 2.88 g (30% yield) of 4-(tert-butyldimethylsilyloxy)-1,6-heptadiene as a transparent colorless...
reference example 2
[0174] The preparation of 4-(triisopropylsilyloxy group)-1,6-heptadiene represented by formula (3)
[0175] To a 50 ml-Schlenk tube was added 1.35 g of imidazole manufactured by Wako Pure Chemical Industries, and then 10 ml of anhydrous N,N-dimethylformamide manufactured by the above company and 1.2 ml of 1 manufactured by Aldrich Chemical Company, 6-Heptadien-4-ol. The resulting mixture was cooled to 0 °C. To this mixture was added 1.93 ml of triisopropylsilyl chloride manufactured by Tokyo Chemical Industry Co., Ltd., and the resulting mixture was stirred at room temperature for 85 hours. An excess of water was then added thereto to terminate the reaction. The product contained in the reaction mixture was extracted with hexane, and the obtained organic extract was dried over anhydrous sodium sulfate manufactured by Nacalai Tesque Inc. Company. The dried hexane solution was vacuum distilled at 93° C. and 21 mmHg to obtain 1.1 g (46 percent yield) of 4-(triisopropylsilyloxy...
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