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A kind of mncoo2/carbon nanotube electrode material and preparation method thereof

A technology of carbon nanotubes and electrode materials, which is applied in the field of electrochemistry and nanomaterials, can solve the problems of failure to meet the basic requirements of supercapacitor electrodes, poor conductivity of manganese cobalt oxides, and low cycle stability, so as to shorten the synthesis time, Improved electrochemical properties and good dispersibility

Active Publication Date: 2018-12-28
SHANGHAI INST OF TECH
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

However, manganese cobalt oxide has poor conductivity and low cycle stability, so it cannot meet the basic requirements of supercapacitor electrodes, which limits its practical application.

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0023] A MnCoO 2 The preparation method of / carbon nanotube and application thereof, comprises the following steps: first with 5mmolKMnO 4 , 1mmolCoSO 4 , 6mmolH 2 SO 4 Put 100ml of deionized water into a three-necked flask, add 0.05g of SDBS, stir at room temperature for 30min, then place in a microwave reactor for reaction, the reaction temperature is controlled at 110°C, and the reaction time is 15min. The product was naturally cooled to room temperature, filtered with suction, and the obtained material was dried at room temperature for 2 days. Secondly, the room temperature activation of carbon nanotubes: respectively soak an appropriate amount of multi-walled carbon nanotube samples in the chromic acid lotion at room temperature, heat and dissolve 2.5g of potassium dichromate in 5ml water, then slowly add 45ml98% vitriol oil, stir at a low speed 10 min, and then diluted with distilled water and then repeatedly washed by suction filtration, the obtained product was heat...

Embodiment 2

[0027] A MnCoO 2 The preparation method of / carbon nanotube and application thereof, comprises the following steps: first with 5mmolKMnO 4 , 5mmolCoSO 4 , 6mmolH 2 SO 4 Put 100ml of deionized water into a three-necked flask, add 0.1g of SDBS, stir at room temperature for 30min, then place in a microwave reactor for reaction, the reaction temperature is controlled at 110°C, and the reaction time is 30min. The product was naturally cooled to room temperature, filtered with suction, and the obtained material was dried at room temperature for 2 days. Secondly, the room temperature activation of carbon nanotubes: respectively soak an appropriate amount of multi-walled carbon nanotube samples in chromic acid lotion at room temperature, heat and dissolve 2.5g potassium dichromate in 5ml water, then slowly add 45ml98% concentrated sulfuric acid, and stir at a low speed for 20min , and then diluted with distilled water and then repeatedly washed by suction filtration, the obtained p...

Embodiment 3

[0031] A MnCoO 2 The preparation method of / carbon nanotube and application thereof, comprises the following steps: first with 5mmolKMnO 4 , 1mmolCoSO 4 , 6mmolH 2 SO 4 Put 100ml of deionized water into a three-necked flask, add 0.2g of SDBS, stir at room temperature for 30min, then place in a microwave reactor for reaction, the reaction temperature is controlled at 110°C, and the reaction time is 45min. The product was naturally cooled to room temperature, filtered with suction, and the obtained material was dried at room temperature for 2 days. Secondly, room temperature activation of carbon nanotubes: respectively soak appropriate amount of multi-walled carbon nanotube samples in chromic acid lotion at room temperature (2.5g potassium dichromate is heated and dissolved in 5ml water, then slowly add 45ml98% concentrated sulfuric acid, stir at low speed 30 min) and then diluted with distilled water and then repeatedly washed by suction filtration, and the obtained product ...

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Abstract

The present invention discloses a MnCoO2 / carbon nanotube electrode material and a preparation method thereof. The method comprises the steps of adopting potassium permanganate as a manganese source, adopting cobalt sulfate as a cobalt source, adopting sodium dodecyl sulfonate (SDBS) as a morphological control agent, and preparing MnCoO2 through the microwave-assisted heating method; soaking a proper amount of a multi-wall carbon nanotube sample in the chromic acid washing liquid to activate the carbon nanotube at the room temperature; finally, mixing MnCoO2 with the activated carbon nanotube,and preparing the MnCoO2 / carbon nanotube electrode material. According to the invention, the electrode material is dried and ground. After that, the material is evenly mixed with carbon black and polytetrafluoroethylene according to a mass ratio, so that the electrode of a super capacitor is prepared. The material disclosed by the invention is environment-friendly, simple in preparation method andconvenient for large-scale production.

Description

technical field [0001] The invention belongs to the technical field of electrochemistry and nanometer materials, in particular to a kind of MnCoO 2 / Carbon nanotube electrode material and preparation method thereof. Background technique [0002] McO 2 It is a manganese-cobalt oxide mainly composed of divalent manganese and divalent cobalt. It has been widely used in electrode materials, magnetic materials, catalysts, environmental treatment, etc., and has become a relatively popular research topic in recent years. The research focus includes its synthesis process and optimization. There are many synthetic methods of manganese cobalt oxides, currently mainly electrochemical method, hydrothermal method, solid phase synthesis method, template method and so on. Using the traditional hydrothermal method to assist in the synthesis of manganese-cobalt oxides, the crystal nucleation process will preferentially occur on the inner wall of the container and on the dust particles, a...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): H01G11/86H01G11/36H01G11/38
Inventor 蒋继波孙瑶馨朱丽莹钱炜陈浩天张小杰常宾靳伟诺杨育涵韩生
Owner SHANGHAI INST OF TECH