Compound and organic electro-luminescent device containing same
A technology of compounds and organic compounds, applied to organic electroluminescent devices, in the field of dibenzoheterocyclic organic compounds of imidazo[1,2-a]pyridine, can solve problems such as unsatisfactory performance and achieve The effect of high luminous efficiency, high electrochemical stability and long device life
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[0051] Synthesis of shared intermediates:
[0052]
[0053] Synthesis of compound 03: To a 2L single-necked bottle, compound 01 (53.17g, 0.57mol, 1.0eq), compound 02 (200g, 0.57mol, 1.0eq), NaHCO 3 (94.9g, 1.14mol, 2.0eq), and isopropanol (1000ml) were put into the flask, heated to about 80 degrees in an oil bath, kept stirring and refluxed for 7 hours, and the reaction of raw materials was monitored by sampling TLC. Cool down, add deionized water dropwise, stir for about 4 hours, and filter with suction. The solid was slurried with ethanol, filtered and dried with suction. 157 g of white solid compound 03 was obtained with a yield of 79.6%. Mass spectrum: 349.03 (M+H)
[0054] Synthesis of Compound 04: Add Compound 03 (60g, 171.81mmol, 1.0eq), bis-pina boronate (56.72g, 223.35mmol, 1.3eq), Pd(dppf)Cl to a 1L single-necked bottle in sequence 2 (1.26g, 1.72mmol, 0.01eq), CH 3 COOK (33.72g, 343.62mmol, 2.0eq), 600ml of dioxane, N2 replacement 3 times under stirring, heat...
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