Lithium-sulfur secondary battery
A lithium-sulfur secondary battery and lithium-sulfur battery technology, applied in secondary batteries, lithium batteries, batteries, etc., can solve problems such as insufficient effect and performance degradation of lithium-sulfur secondary batteries, and achieve high energy density
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Embodiment 1
[0185] In ethanol (200mL), sulfur (S 8 ) (38 g) and iron phthalocyanine (FePc, product of Sigma-Aldrich Company) (150 mg) as catalytic sites were mixed, and the resultant was ball-milled for 3 hours to prepare iron phthalocyanines having been introduced as catalytic sites. (FePc) of sulfur (FePc-S).
[0186] Subsequently, carbon nanotubes (product of CNanoTechnology Co., Ltd.) (13.5 g) were added to the catalytic site-introduced sulfur (FePc—S) prepared above, and the resultant was ball milled for 3 hours to obtain a mixture.
[0187] Then, the above-prepared mixture was filtered with a vacuum pump, and then washed with ethanol (1000 mL), and the upper layer powder of the mixture obtained from the filtration and washing was dried at 80° C. for 12 hours to prepare a sulfur-carbon mixture.
[0188] Subsequently, the sulfur-carbon mixture prepared above was placed in an oven at 155° C. for 30 minutes for composite formation, and a sulfur-carbon composite material (S / C 70:30 weig...
experiment example 1
[0213] Experimental example 1. Performance evaluation of lithium-sulfur secondary battery
[0214] The performance of each lithium-sulfur secondary battery manufactured in Examples and Comparative Examples was evaluated using a charge-discharge measuring device (LAND CT-2001A, Wuhan, China).
[0215] For each lithium-sulfur secondary battery, at 0.1C (0.55mA·cm -2 ) charging / 0.1C(0.55mA·cm -2 ) discharge for 2.5 cycles, and then at 0.2C (1.1mA·cm -2 ) charging / 0.2C(1.1mA·cm -2 ) discharge for 3 cycles, and then at 0.3C (1.65mA·cm -2 ) charging / 0.5C(2.65mA·cm -2 ) discharge, three measurements were carried out at 25°C. The results obtained here are shown in Table 2 and figure 2 middle.
[0216] [Table 2]
[0217]
[0218] Such as figure 2 As shown, it was confirmed that, compared with Comparative Example 1, the lithium-sulfur secondary battery including the positive electrode according to the present invention had more excellent discharge capacity and overvoltage ...
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