The invention belongs to the technical field of traditional Chinese medicines, and relates to a traditional Chinese medicine package for treating cardiovascular and cerebrovascular diseases by smell and a preparation method of the traditional Chinese medicine package. The traditional Chinese medicine package includes the following raw materials in parts by weight: 20-40 parts of sandalwood, 20-40parts of storax, 20-40 parts of rhizoma kaempferiae, 15-25 parts of ramulus cinnamomi, 10-20 parts of camphor, 5-15 parts of borneol, and 1-5 parts of musk; and a use method uses a smell administration manner, and includes the following steps: putting the traditional Chinese medicine package into a smell rehabilitation training device, wearing a breathing device of the smell rehabilitation training device by a user, starting a switch on the smell rehabilitation training device, and allowing traditional Chinese medicine gas in the smell rehabilitation training device to realize the effect through nasal mucosa absorption or immune response of olfactory cells. The traditional Chinese medicine package for treating the cardiovascular and cerebrovascular diseases adopts smell therapy, has obvious effects on reducing hyperlipidemia, coronary heart disease and high blood pressure, has the functions of passing aroma, inducing resuscitation and restoring consciousness, promoting qi circulation to relieve pain, and warming channels and supporting yang, and is used for chest distress, chest pain, dizziness, nausea, coronary heart disease and angor pectoris.