Compound separated from gamboge resin and derivative thereof and pharmaceutical composition comprising compound and derivative
A compound, technology from Garcinia cambogia, applied in the field of novel compounds and their derivatives
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Embodiment 1
[0244] Example 1. Analytical grade (analytical) reversed phase high performance liquid chromatography (reversed phase high performance liquid chromatography, RP-HPLC) analysis of the acetone extraction product TSB-14 of garcinia resin
[0245] This experiment mainly analyzes the acetone extraction product TSB-14 of gamboge resin obtained in Example 1 of a Taiwan patent case TW I282280 (corresponding to US7,138,428 B2 and CN 100413868 C) of the applicant. Grade RP-HPLC, in order to further confirm that the acetone extraction product TSB-14 of garcinia resin contains those components.
[0246] The acetone extraction product TSB-14 of the garcinia cambogia resin of 1.0 mg was dissolved in 1 mL of acetone, and carried out analytical grade RP-HPLC according to the method described in the "general operating procedure" above, and obtained as figure 1 Analytical RP-HPLC elution profile shown.
[0247] From figure 1 It can be seen that the acetone extraction product TSB-14 of garci...
Embodiment 2
[0248] Example 2. Preparation of Purified Compounds Derived from Acetone Extracted Products of Garcinia Resin
[0249] The semi-preparative grade RP-HPLC of the acetone extraction product TSB-14 of A, garcinia resin:
[0250] The acetone extraction product TSB-14 of 3 g of garcinia resin was dissolved in 30 mL of acetone / acetonitrile (v / v=1:9), and the semi-preparative RP- HPLC, wherein the mobile phase is 0.05% TFA aqueous solution / 65% acetonitrile=35:65. The resulting semi-prep RP-HPLC elution profile is shown in figure 2 middle. Will figure 2 with the above embodiment 1 figure 1 After a comparison, it can be clearly seen that the peaks 1 to 35 are in the figure 2 s position. The applicant divides these 35 peaks into 3 sections (sections) (that is, section 1 to section 3), wherein section 1 contains peaks 1 to 12, and the residence time is from the 0th to the 42nd minute; Section 2 contains peaks 13 to 24 with residence times from 42 to 135 minutes; and section 3 ...
Embodiment 3
[0273] Example 3. Characterization of Compounds Purified from Fraction 1 to Fraction 3
[0274] The 35 products derived from the separation part 1 to the separation part 3 obtained in the above Example 2 were analyzed according to the method described in the above "general operating procedure" for physical and chemical properties, including melting point, 1H-NMR, 13C -NMR, homonuclear correlation spectroscopy (1H-1H COZY), heteronuclear multiple-quantum coherence (HMQC), heteronuclear multiple-bond coherence (HMBC), nuclear Overhauser Effect spectroscopy (nuclearOverhauser effect spectroscopy, NOESY), EIMS, HREIMS, FABMS and HRFABMS. The experimental data obtained are summarized as follows:
[0275] 1. Product Gh-47:
[0276] The measured properties of the product Gh-47 are as follows:
[0277] Yellow flaky crystal, melting point: 204-209°C.
[0278] EIMS m / z (relative intensity): 560[M]+(100), 545(47), 532(22), 517(36), 405(44), 389(11), 363(24), 349( 17), 307(12), 287(2...
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