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Preparation method and application of photoelectric aptamer sensor based on ppy/cds/g‑c3n4

An aptamer sensor, g-c3n4 technology, applied in instruments, scientific instruments, material analysis through electromagnetic means, etc., to achieve high-sensitivity detection, simple operation, and wide signal response range

Active Publication Date: 2018-01-16
上海佑科仪器仪表有限公司
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

However, due to the high electron-hole recombination efficiency under illumination, g-C 3 N 4 There are still some limitations in practical applications

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0027] Example 1 A based on PPy / CdS / g-C 3 N 4 Preparation method of photoelectric aptasensor

[0028] (1) Pretreatment of the ITO electrode: cut the ITO conductive glass to a size of 1.0 cm × 2.5 cm, clean it with detergent, acetone, ethanol and ultrapure water for 30 min, and dry it with nitrogen;

[0029] (2) Add 6 µL, 3 mg / mL polypyrrole sensitized cadmium sulfide / carbon nitride PPy / CdS / g-C dropwise 3 N 4 The solution is placed on the surface of the electrode and dried at room temperature;

[0030] (3) Add 6 μL, 1 μmol / L aptamer solution dropwise to the surface of the electrode, dry it in a refrigerator at 4°C, and rinse with Tris-HCl buffer;

[0031] (4) Drop 6 µL, 1 mmol / L 6-mercaptohexanol solution on the surface of the electrode to seal the non-specific active sites on the surface of the electrode, and dry it in a refrigerator at 4°C;

[0032] (5) Rinse with Tris-HCl buffer solution, let it dry to a wet state, add 6 μL of adenosine solutions with different concentr...

Embodiment 2

[0033] Example 2 A PPy / CdS / g-C based 3 N 4 Preparation method of photoelectric aptasensor

[0034] (1) Pretreatment of the ITO electrode: cut the ITO conductive glass to a size of 1.0 cm × 2.5 cm, clean it with detergent, acetone, ethanol and ultrapure water for 30 min, and dry it with nitrogen;

[0035] (2) Add 6 µL, 4 mg / mL polypyrrole sensitized cadmium sulfide / carbon nitride PPy / CdS / g-C dropwise 3 N 4 The solution is placed on the surface of the electrode and dried at room temperature;

[0036] (3) Add 6 μL, 0.5 μmol / L aptamer solution dropwise to the surface of the electrode, dry it in a refrigerator at 4°C, and rinse with Tris-HCl buffer;

[0037] (4) Add 6 µL, 2 mmol / L 6-mercaptohexanol solution dropwise on the electrode surface to seal the non-specific active sites on the electrode surface, and dry it in a refrigerator at 4°C;

[0038] (5) Rinse with Tris-HCl buffer solution, let it dry to a wet state, add 6 μL of adenosine solutions with different concentrations ...

Embodiment 3

[0039] Example 3 A PPy / CdS / g-C based 3 N 4 Preparation method of photoelectric aptasensor

[0040] (1) Pretreatment of the ITO electrode: cut the ITO conductive glass to a size of 1.0 cm × 2.5 cm, clean it with detergent, acetone, ethanol and ultrapure water for 30 min, and dry it with nitrogen;

[0041] (2) Add dropwise 6 µL, 5 mg / mL polypyrrole-sensitized cadmium sulfide / carbon nitride PPy / CdS / g-C 3 N 4 The solution is placed on the surface of the electrode and dried at room temperature;

[0042] (3) Add 6 μL, 1.5 μmol / L aptamer solution dropwise on the surface of the electrode, dry it in a refrigerator at 4°C, and rinse with Tris-HCl buffer;

[0043] (4) Add 6 µL, 3 mmol / L 6-mercaptohexanol solution dropwise on the surface of the electrode to seal the non-specific active sites on the surface of the electrode, and dry it in a refrigerator at 4°C;

[0044] (5) Rinse with Tris-HCl buffer solution, let it dry to a wet state, add 6 μL of adenosine solutions with different c...

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PUM

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Abstract

The invention relates to a preparation method and application of a PPy / CdS / g-C3N4 based photoelectric adapter sensor and belongs to the technical field of novel functional materials and biological sensing detection. Specifically, a photoelectric active substance PPy / CdS / g-C3N4 is modified on the surface of conductive glass, an unmarked type photoelectric adapter sensor is prepared, and rapid and ultra-sensitive detection of adenosine molecules is achieved.

Description

technical field [0001] The present invention relates to a kind of based on PPy / CdS / g-C 3 N 4 Preparation method and application of photoelectric aptasensor. Specifically, modify the photoelectric active material PPy / CdS / g-C on the surface of conductive glass 3 N 4 , to prepare a label-free optoelectronic aptasensor for rapid and ultrasensitive detection of adenosine molecules. The invention belongs to the technical field of new functional materials and biosensing detection. Background technique [0002] In recent years, photoelectrochemical analysis has attracted more and more attention. In the photoelectrochemical detection process, light is the excitation signal, and the resulting photocurrent is the detection signal. Compared with traditional electrochemical analysis, photoelectrochemical analysis has higher sensitivity due to the complete separation of excitation signal and detection signal. In addition, compared with the complex and expensive optical detection de...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): G01N27/327G01N27/416
CPCG01N27/3275G01N27/416
Inventor 魏琴孙旭吴丹马洪敏范大伟胡丽华
Owner 上海佑科仪器仪表有限公司