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Process for the separation of diethylbenzene in carbon deka-aromatic hydrocarbons

A carbon ten aromatic hydrocarbon and separation method technology, applied in the field of separation of diethylbenzene, can solve the problems of not finding an efficient adsorbent desorbent, large investment, etc., and achieve good separation effect and thermal stability, low energy consumption, and product purity. high effect

Active Publication Date: 2011-04-20
PETROCHINA CO LTD
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

The advantages of the adsorption method are outstanding, that is, stable operation and high product purity; the disadvantage is that the investment is large, and no efficient adsorbent and corresponding desorbent have been found.

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0013] 1.C 10 Preliminary Separation of Mixed Diethylbenzene in Heavy Aromatics

[0014] to C 10 The heavy aromatics reformate feedstock is subjected to initial fractionation to separate the diethylbenzene component. Some main parameters of the rectification experimental device: rectification column type: packed column, with vacuum sleeve for heat insulation; packing material: 2mm θ ring; rectification column size: 30mm×1.5m; kettle capacity: 3000ml; The way of distillation, normal pressure operation. Heating and distilling the raw materials in the tower kettle, a condenser is installed at the top of the tower, and the reflux ratio is controlled by a reflux ratio controller. At the beginning, use full reflux and heat quickly to make the liquid in the tower kettle boil quickly. After the reflux liquid is present at the top of the tower, reduce the heating power of the tower kettle to make the temperature at the top of the tower and reflux stable. The weight ratio of reflux t...

Embodiment 2

[0022] 1.C 10 Preliminary Separation of Mixed Diethylbenzene in Heavy Aromatics

[0023] The rectification experimental apparatus is identical with embodiment 1. The weight ratio of reflux to outflow was 3:1, and the production rate was 30 g / h. The fraction in the range of 178-182° C. was collected, and the mixed diethylbenzene content was 84.2% by weight. 2. Extractive distillation

[0024] The extractive distillation experimental device is the same as in Example 1. The extractant is dibutyl phthalate: the flow rate is 300 g / hour. Feed temperature ~ 180 ° C, feed position is the upper half of the tower; raw material concentration: mixed diethylbenzene content is 84.2% (weight)), flow rate 60 grams / hour, feed temperature 150 ° C, feed position is extraction The lower half of the distillation column.

[0025] A mixture of extractant, p-diethylbenzene and a small amount of m-diethylbenzene flows out from the bottom of the column. Meta-diethylbenzene is condensed by the ...

Embodiment 3

[0029] 1.C 10 Preliminary Separation of Mixed Diethylbenzene in Heavy Aromatics

[0030] The rectification experimental apparatus is identical with embodiment 1. The weight ratio of reflux to outflow was 30:1 and the production rate was 30 g / h. The fractions in the range of 178-182° C. were collected, and the separated mixed diethylbenzene content was 92.5% by weight.

[0031] 2. Extractive distillation

[0032] The extractive distillation experimental device is the same as in Example 1. The extractant is a mixture of dimethyl phthalate and dibutyl phthalate, the weight ratio is 1:1: the flow rate is 800 g / hour. Feed temperature ~ 180°C, feed position is the upper half of the tower; raw material concentration: mixed diethylbenzene 92.5% (weight), flow rate 40 g / h, feed temperature 150°C, feed position is the extractive distillation column lower half.

[0033]A mixture of extractant, p-diethylbenzene and a small amount of m-diethylbenzene flows out from the bottom of the ...

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Abstract

The invention relates to a method for utilizing an extractive distillation process to separate diethyl benzene from C10 arene, comprising: firstly, mixed components of meta-diethyl benzene in C10 arene and other high boiling point components are separated off, with a rectification temperature of between 176 and 182DEG C; then an extractant is added in a meta-diethyl benzene mixture for separating out m-diethyl benzene, wherein, the extractant is dimethyl phthalate, dibutyl phthalate or a mixture thereof; and the extractant and the mixed components of meta-diethyl benzene have a feeding weight ratio of 5 to 20:1, the charging temperature of the extractant is between 120 and 190 DEG C, and the separation temperature is 160 to 190 DEG C; and finally the extractant and the p-diethyl benzene are separated for recovering the extractant through distillation separation; and the method has advantages of simple process, stable operation, low energy consumption, high purity of separated products, good separation effect and thermal stability of extractant, economy and acquirability, and the p-diethyl benzene content can reach over 98 percent, and the m-diethyl benzene content can reach above 70 percent.

Description

technical field [0001] The invention relates to a method for separating diethylbenzene from carbon ten aromatic hydrocarbons by means of extractive distillation. Background technique [0002] With the continuous development of the oil refining industry, wide-fraction catalytic reforming unit C from polyester raw material plants 10 The amount of heavy aromatics is also increasing significantly, and the development of heavy aromatics separation technology is becoming more and more important. Especially for Accounting C 10 The separation technology of about 12% diethylbenzene in the raw material needs to be further improved. Although C 10 The composition of heavy aromatics is very complex, and the content of each component changes continuously with the change of its production process parameters and actual operation conditions, but its main components and their content are basically stable, also C 10 The separation, purification and comprehensive utilization of heavy aromat...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C07C15/02C07C7/04C07C7/10
Inventor 刘键杜建卫黄奋生张卫星陈季敏
Owner PETROCHINA CO LTD