Photosensitive resin composition
A technology of photosensitive resin and composition, which is applied in the field of photosensitive resin composition, and can solve problems such as longer exposure time, increased number of steppers, and low sensitivity
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[0241] Hereinafter, the present invention will be described based on reference examples and working examples. The evaluation of the photosensitive resin composition in an Example was performed by the following method.
[0242]
[0243] (1) Evaluation of patterning characteristics
[0244] With a spin coater (Dspin SW-636, manufactured by DAINIPPON SCREEN MFG.CO., LTD.), the photosensitive resin composition is spin-coated on a 5-inch silicon wafer, and prebaked at 125°C for 180°C on a hot plate. Seconds, a coating film with a film thickness of 9.0 μm was formed. The coating film was heat-treated (cured) at 320° C. for 1 hour in a nitrogen atmosphere using a temperature-rising programmable curing furnace (VF-2000 type, manufactured by Koyo Thermo Systems Co., Ltd.) to obtain a cured film on a silicon wafer . The film thickness was measured with an optical film thickness measuring device (LAMBDA-ACE VM-1200, manufactured by DAINIPPON SCREEN MFG.CO., LTD.) at a refractive ind...
reference example 1
[0257]In a separable flask with a capacity of 2L, 197.8g (0.54mol) of 2,2-bis(3-amino-4-hydroxyphenyl)-hexafluoropropane, 75.9g (0.96mol) of pyridine and 692g of DMAc were placed at room temperature Mix and dissolve with stirring at 25 °C. Separately, a solution obtained by dissolving 19.7 g (0.12 mol) of 5-norbornene-2,3-dicarboxylic anhydride in 88 g of DMDG was dropped into the above-mentioned flask through the dropping funnel. The time required for the dropwise addition was 40 minutes, and the maximum temperature of the reaction solution was 28°C.
[0258] After the dropwise addition, it was heated to 50°C in a hot water bath and stirred for 18 hours. Then, the IR spectrum of the reaction solution was measured, and it was confirmed that a 1385cm -1 and 1772cm -1 The characteristic absorption of the imino group.
[0259] Then, the reaction solution was cooled to 8° C. with a water bath, and a solution obtained by dissolving 142.3 g (0.48 mol) of 4,4’-diphenyl ether dicar...
reference example 2
[0265] In Reference Example 1, 125.35 g (0.48 mol) of octahydro-1H-4,7-methyleneindene dicarboxylic acid dichloride was used instead of 142.3 g (0.48 mol) of 4,4'-diphenyl ether dicarboxylic acid acid dichloride, and 139.45 g (0.54 mol) of 2,2-bis(3-amino-4-hydroxyphenyl)-propane was used instead of 197.8 g (0.54 mol) of 2,2-bis(3-amino-4- A polybenzoxazole resin precursor (P-2) was obtained in exactly the same manner as in Reference Example 1 except that hydroxyphenyl)-hexafluoropropane. The polystyrene conversion weight average molecular weight of this resin was 22000 (Mw).
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