Active malodor eliminator with low volatility and its use
A technology for eliminating agents and odors, applied in disinfection, deodorization, organic chemical methods, etc.
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Embodiment 1
[0068] Embodiment 1: the preparation of levulinic acid chloride
[0069]
[0070] Oxalyl chloride (2M, 450ml, 0.9mol) in dichloromethane was added dropwise to stirring of levulinic acid (100g, 0.857mol) and dimethylformamide (DMF, 2ml) over about 1.5 to 2 hours at room temperature. in the mixture. After the addition was complete, the resulting mixture was stirred for an additional 0.5 h. The solvent was removed in vacuo and the crude mixture was used in the subsequent reaction.
Embodiment 2
[0071] Embodiment 2: Preparation of acetylacetonate (Levulinic TETRONICS) (compound 2)
[0072] Triethylamine (6.91ml, 49.50mmol) was added to a stirred mixture of Tetron 901 (23.5g, 24.77mmol) in dichloromethane (150ml) under nitrogen atmosphere at 0-5°C. Then levulinic acid chloride (prepared in Example 1) was added dropwise. The resulting mixture was warmed to room temperature and stirred overnight. Triethylammonium chloride was then filtered off. The organic layer was washed with saturated Na 2 CO3 Washed and concentrated in vacuo to obtain >90% functionalized product tetraketone levulinate as determined by NMR spectroscopy.
Embodiment 3
[0073] Embodiment 3: Preparation of levulinate MALTRIN QD M585 maltodextrin (Levulinate MALTRIN QD M585 Maltodextrin)
[0074] Triethylamine (12.5 g, 0.124 mmol) was added to a stirred mixture of MALTRIN QD M585 maltodextrin (16.2 g, 0.100 mol) dissolved in DMF (60 ml) under a nitrogen atmosphere at 0-5°C. The molar ratio of maltodextrin here is based on the monomer molecular structure of the entire polymer chain. Then levulinic acid chloride (prepared in Example 1) was added dropwise. The resulting mixture was warmed to room temperature and stirred overnight. Triethylammonium chloride was then filtered off. The precipitate was collected with tetrahydrofuran (THF) / isopropanol (IPA) in a volume ratio of 1:9 (THF:IPA). The solid was filtered, washed several times with a THF:IPA mixture, and dried under vacuum to obtain the product MALTRIN QDM585 maltodextrin levulinate approximately 15-20% functionalized by NMR spectroscopy.
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