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Polyvinyl butyral preparation method

A technology of polyvinyl butyral and polyvinyl alcohol, applied in the field of polymer chemistry, can solve the problems of poor thermal stability of PVB film strength polyvinyl butyral, etc., and achieve the effect of significant technological progress

Inactive Publication Date: 2015-10-28
宜春市康盛高分子材料科技有限公司
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0005] Aiming at the above-mentioned technical problems in the prior art, the invention provides a kind of preparation method of polyvinyl butyral, the preparation method of described this polyvinyl butyral should solve the preparation method in the prior art to obtain The low butyraldehyde group value in polyvinyl butyral affects the strength of PVB film and the technical problems of poor thermal stability of polyvinyl butyral

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0019] Add 6000kg of deionized water into a 10000L (10T) enamel reaction kettle with a stirring, heating and dropping system, add 750kg of polyvinyl alcohol under stirring at 80r / min, and raise the temperature to 95±1°C. Dissolve polyvinyl alcohol (PVA) in 4 hours, then, when the dissolved PVA is cooled to 20±2°C, add 1500 kg of hydrochloric acid solution with a mass percent solubility of 2.5% in 30 minutes, and cool to 10±2°C after adding the acid 2°C, first drop 300kg of n-butyraldehyde into the acidic PVA solution; the dropping time is 40min; the stirring speed is 150r / min; Next, add the remaining 150kg of n-butyraldehyde dropwise in 30min. After adding n-butyraldehyde dropwise, keep the reaction at 10±2°C for 60 minutes; then, heat it to 64±1°C at a heating rate of 10°C / h, and keep it at this temperature for 90 minutes. After the reaction, the reaction mass was cooled to 30°C. The material PVB is moved to the centrifuge for dehydration, so that the moisture content is le...

Embodiment 2

[0023] Add 6000kg of deionized water into a 10000L (10T) enamel reaction kettle with a stirring, heating and dropping system, add 750kg of polyvinyl alcohol under stirring at 80r / min, and raise the temperature to 95±1°C. Dissolve polyvinyl alcohol (PVA) in 4 hours, then, when the dissolved PVA is cooled to 20±2°C, add 1500 kg of hydrochloric acid solution with a mass percent solubility of 2.5% in 30 minutes, and cool to 10±2°C after adding the acid 2°C, first drop 300kg of n-butyraldehyde into the acidic PVA solution; the dropping time is 40min; the stirring speed is 150r / min; Next, add the remaining 150kg of n-butyraldehyde dropwise in 30min. After adding n-butyraldehyde dropwise, keep the reaction at 10±2°C for 60 minutes; then, heat it to 64±1°C at a heating rate of 10°C / h, and keep it at this temperature for 90 minutes. After the reaction, the reaction mass was cooled to 30°C. The material PVB is moved to the centrifuge for dehydration, so that the moisture content is le...

Embodiment 3

[0027] Add 6000kg of deionized water into a 10000L (10T) enamel reaction kettle with a stirring, heating and dropping system, add 750kg of polyvinyl alcohol under stirring at 80r / min, and raise the temperature to 85±2°C. Dissolve polyvinyl alcohol (PVA) in 4 hours, then, when the dissolved PVA is cooled to 20±2°C, add 1500 kg of hydrochloric acid solution with a mass percent solubility of 2.5% in 30 minutes, and cool to 10±2°C after adding the acid 2°C, first drop 300kg of n-butyraldehyde into the acidic PVA solution; the dropping time is 40min; the stirring speed is 150r / min; Next, add the remaining 150kg of n-butyraldehyde dropwise in 30min. After adding n-butyraldehyde dropwise, keep the reaction at 10±2°C for 60 minutes; then, heat it to 64±1°C at a heating rate of 10°C / h, and keep it at this temperature for 90 minutes. After the reaction, the reaction mass was cooled to 30°C. The material PVB is moved to the centrifuge for dehydration, so that the moisture content is le...

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Abstract

The present invention relates to a polyvinyl butyral preparation method, which comprises: adopting polyvinyl alcohol with an alcoholysis degree of 97.0-98.5% as a raw material, dissolving with deionized water, cooling, carrying out a reaction of the polyvinyl alcohol and one part of butyraldehyde at a low temperature under catalysis of an inorganic acid, adding the remaining butyraldehyde to continuously react with the polyvinyl alcohol, heating to a temperature of 50-70 DEG C in a heating rate of 8-12 DEG C / h so as to achieve complete acetalation, separating the polyvinyl butyral and the acid liquid through a centrifuge after completing the reaction, washing the separated polyvinyl butyral with deionized water and an dilute alkali solution in a vacuum suction filtration washing machine, and carrying out centrifuged drying and flash drying to obtain the polyvinyl butyral. According to the present invention, the thermal stability test results show that the PVB does not yellow within 1.5 h at the high temperature of 180 DEG C, the butyraldehyde group value (%) is more than 76, the hydroxyl value (%) is more than 18-19.5, and the haze (%) is less than 0.3.

Description

Technical field: [0001] The invention belongs to the field of macromolecular chemistry, and in particular relates to a polyvinyl butyral, specifically a preparation method of polyvinyl butyral. technical background: [0002] Polyvinyl butyral is formed by condensation of polyvinyl alcohol (PVA) and n-butyraldehyde in aqueous solution through inorganic acid-catalyzed condensation. It is a thermoplastic polymer compound, referred to as PVB. [0003] With the continuous development of my country's national economy, the use of PVB has gradually entered a wider range of fields. Especially with the rapid development of my country's automobile industry and the Ministry of Construction's strict safety requirements for high-rise building glass, the domestic market demand for PVB has increased significantly every year. However, because domestic PVB preparation technology still has a certain gap compared with foreign countries, high-quality PVB needs to be imported in large quantities...

Claims

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Application Information

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Patent Type & Authority Applications(China)
IPC IPC(8): C08F16/06C08F8/28
Inventor 金东元杨志强
Owner 宜春市康盛高分子材料科技有限公司