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A kind of precursor preparation method of platinum series catalyst

A platinum-based catalyst and precursor technology, which is applied in the field of platinum-based catalyst precursor preparation, can solve the problems of increasing catalyst preparation cost, cumbersome cleaning steps, etc., and achieves the effect of improving the utilization rate of catalytic rate, rational distribution and combination, and simple process

Active Publication Date: 2018-04-13
上海河森电气有限公司
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

At the same time, if the anion of the prepared catalyst precursor contains SO 4 2- , NO 3 - , then cumbersome cleaning steps are required in the catalyst preparation process, which will greatly increase the preparation cost of the catalyst

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0034] Commercially available [Pt(NH 3 ) 4 ]Cl 2 Dissolve in deionized water and configure a solution with a mass concentration of 1%, place 110 grams of commercially available DuPont Nafion211 membrane (H type) in the solution, carry out ion exchange under normal temperature conditions, and the immersion time is 12h; containing [Pt(NH 3 ) 4 ] 2+ The ionized Nafion211 membrane was washed repeatedly with deionized water, dried in the shade, and immersed in 0.5% H 2 C 2 o 4 In the ethanol solution, ion exchange was carried out at room temperature, and the immersion time was 12 hours; after the immersion was completed, the solution was filtered, the white precipitate was collected, and dried under reduced pressure at 90°C to obtain a precursor without CL-platinum catalyst White powder; The 0.726g white powder that will make is dissolved in 10ml deionized water and is made into solution, and adds the commercially available carbon black carrier of 0.6g (the catalyst carrier ...

Embodiment 2

[0036] Commercially available [Pt(NH 3 ) 4 ]Cl 2 Dissolve in deionized water and configure a solution with a mass concentration of 1%, place 110 grams of commercially available DuPont Nafion211 membrane (H type) in the solution, carry out ion exchange under normal temperature conditions, and the immersion time is 12h; containing [Pt(NH 3 ) 4 ] 2+ The ionized Nafion211 membrane was washed repeatedly with deionized water, dried in the shade, and immersed in CH with a mass concentration of 0.5%. 3In the COOH ethanol solution, ion exchange was carried out at room temperature, and the immersion time was 12 hours; after the immersion was completed, the solution was filtered, the white precipitate was collected, and dried under reduced pressure at 90°C to obtain a precursor without CL-platinum catalyst body white powder; the prepared 0.783g white powder is dissolved in 10ml deionized water to form a solution, and the commercially available carbon black carrier of 0.6g is added i...

Embodiment 3

[0038] Commercially available [Pt(NH 3 ) 4 ] Cl 2 Dissolve in deionized water and configure a solution with a mass concentration of 1%, place 110 grams of commercially available DuPont Nafion211 membrane (H type) in the solution, carry out ion exchange under normal temperature conditions, and the immersion time is 12h; containing [Pt(NH 3 ) 4 ] 2+ The ionized Nafion211 membrane was washed repeatedly with deionized water, dried in the shade, and immersed in NaHCO with a mass concentration of 0.5%. 3 In the ethanol solution, ion exchange was carried out at room temperature, and the immersion time was 12 hours; after the immersion was completed, the solution was filtered, the white precipitate was collected, and dried under reduced pressure at 90°C to obtain a precursor without CL-platinum catalyst White powder; The 0.798g white powder that will make is dissolved in 10ml deionized water and is made into solution, and adds the commercially available carbon black carrier of 0....

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Abstract

The present invention relates to a platinum catalyst precursor preparation method. According to the method, a cation exchange resin is used as the carrier of the preparation process, a two-step ion exchange method is used, and a carbon black is adopted as the carrier to prepare the platinum catalyst precursor being not contain Cl<->, SO4<2-> and NO3<->. Compared with the method in the prior art, the method of the present invention has characteristics of simple preparation process, no environmental pollution, and low production cost.

Description

technical field [0001] The invention belongs to the technical field of fuel cells, and relates to a method for preparing a precursor of a platinum series catalyst. Background technique [0002] At present, in the field of fuel cells, proton exchange membrane fuel cells (PEMFC) have become a technology researched and developed by many countries in the world. PEMFC fuel cell electrodes usually use solid proton exchange membranes as electrolytes, and catalysts such as platinum are sprayed on the negative and positive sides of the membrane or membrane support layer to form MEA (membrane electrode assembly). [0003] This type of electrode with catalysts such as platinum can react fuels such as hydrogen, methanol, etc., with oxygen directly at the cathode and anode of the electrode, and the electrode will generate electricity, and the discharge will be H 2 O. The conversion efficiency of the fuel cell is relatively high, generally up to 50%, which is much higher than that of th...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): B01J23/42
Inventor 黄启华贾国忠
Owner 上海河森电气有限公司