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A low-temperature proton conductor solid oxide electrolytic cell

A solid oxide, proton conductor technology, applied in the direction of electrolysis components, electrolysis process, electrodes, etc., can solve the problems of high cost, difficult utilization of waste heat, high operating temperature, and achieve the effect of reducing temperature

Active Publication Date: 2019-03-12
DALIAN INST OF CHEM PHYSICS CHINESE ACAD OF SCI
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  • Summary
  • Abstract
  • Description
  • Claims
  • Application Information

AI Technical Summary

Problems solved by technology

[0005] For traditional zirconia-based electrolytic cells, the operating temperature is high, the cost is high, and it is not easy to combine with waste heat utilization, etc.

Method used

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Examples

Experimental program
Comparison scheme
Effect test

Embodiment 1

[0021] Using NiO and BaCe 0.6 Zr 0.25 Y 0.15 o 3-δ , mixed at a weight ratio of 50:50, prepared a 0.5 mm thick hydrogen electrode substrate by dry pressing, and sintered at 1400 ° C for 4 hours to obtain a hydrogen electrode; coated with a layer containing BaCe 0.6 Zr 0.25 Y 0.15 o 3-δ A slurry with a thickness of 20 μm was sintered at 1600 °C for 2 h to obtain a hydrogen electrode / electrolyte assembly; the BaCe 0.6 Zr 0.25 Y 0.15 o 3-δ and BaCo 0.4 Fe 0.4 Zr 0.1 Y 0.1 o 3-δ After mixing at a weight ratio of 30:70, an oxygen electrode was prepared by screen printing, and sintered at 1000°C for 2 hours to obtain an electrolytic cell.

[0022] The electrochemical performance of the solid oxide electrolytic cell was tested using an electrochemical workstation. The performance test results of the solid oxide electrolytic cell show that at 600°C, 50ml / min of water vapor is passed through, and 0.4A / cm can be generated at an electrolytic voltage of 1.25V. 2 the electr...

Embodiment 2

[0024] Using NiO and BaCe 0.6 Zr 0.25 Y 0.15 o 3-δ , mixed at a weight ratio of 70:30, a 1.5 mm thick hydrogen electrode substrate was prepared by dry pressing, and sintered at 1200 ° C for 4 hours to obtain a hydrogen electrode; a layer containing BaCe 0.6 Zr 0.25 Y 0.15 o 3-δ A slurry with a thickness of 50 μm was sintered at 1700 °C for 2 h to obtain a hydrogen electrode / electrolyte assembly; the BaCe 0.6 Zr 0.25 Y 0.15 o 3-δ and BaCo 0.2 Fe 0.5 Zr 0.2 Y 0.1 o 3-δ After mixing at a weight ratio of 10:90, an oxygen electrode was prepared by screen printing, and sintered at 1400°C for 2 hours to obtain an electrolytic cell.

[0025] The electrochemical performance of the solid oxide electrolytic cell was tested using an electrochemical workstation. The performance test results of the solid oxide electrolytic cell show that at 400°C, 50ml / min water vapor can be introduced, and 0.3A / cm can be generated at an electrolytic voltage of 1.5V. 2 the electrolysis curre...

Embodiment 3

[0027] Using NiO and BaCe 0.6 Zr 0.25 Y 0.15 o 3-δ , after mixing at a weight ratio of 30:70, a hydrogen electrode substrate with a thickness of 1 mm was prepared by dry pressing, and sintered at 1200 ° C for 4 hours to obtain a hydrogen electrode; a layer containing BaCe was coated on it 0.6 Zr 0.25 Y 0.15 o 3-δ A slurry with a thickness of 10 μm was sintered at 1400 °C for 2 h to obtain a hydrogen electrode / electrolyte assembly; the BaCe 0.6 Zr 0.25 Y 0.15 o 3-δ and BaCo 0.4 Fe 0.2 Zr 0.3 Y 0.1 o 3-δ After mixing at a weight ratio of 40:60, an oxygen electrode was prepared by screen printing, and sintered at 1200°C for 2 hours to obtain an electrolytic cell.

[0028] The electrochemical performance of the solid oxide electrolytic cell was tested using an electrochemical workstation. The performance test results of the solid oxide electrolytic cell show that at 300°C, 50ml / min water vapor can be introduced, and 0.2A / cm can be generated at an electrolytic voltag...

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Abstract

The invention relates to a low-temperature proton conductor solid oxide electrolytic cell, which includes an electrolyte, a hydrogen electrode and an oxygen electrode, wherein the hydrogen electrode is composed of: NiO and BaCe0.6Zr0.25Y0.15O3-δ; the oxygen The electrode composition is: BaCe0.6Zr0.25Y0.15O3-δ and BaCoaFebZrcYdO3-δ, wherein, 0≤a≤0.5, 0≤b≤0.5, 0≤c≤0.4, 0≤d≤0.4. The proton conductor electrolyte material is: BaCe0.6Zr0.25Y0.15O3-δ. The proton conductor solid oxide electrolytic cell has high water electrolytic activity under the condition of low temperature (300-600 DEG C).

Description

technical field [0001] The invention relates to a solid oxide electrolytic cell, in particular to a low-temperature proton conductor solid oxide electrolytic cell. BaCe, a proton conductor material with high conductivity under low temperature (300-600°C) conditions 0.6 Zr 0.25 Y 0.15 o 3-δ As an electrolyte material, the high oxygen evolution active material BaCo a Fe b Zr c Y d o 3-δ As an oxygen electrode material, realize the high water electrolysis performance of the solid oxide electrolysis cell at a low temperature of 300-600 ° C. The improvement of the low temperature water electrolysis performance is of great significance for promoting the development of the solid oxide fuel electrolysis cell technology to the application technology. . Background technique [0002] Hydrogen energy is considered as the most potential energy carrier in the future due to its clean and efficient characteristics. Solid oxide electrolysis cells (SOEC) is a high-efficiency, low-po...

Claims

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Application Information

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Patent Type & Authority Patents(China)
IPC IPC(8): C25B11/04C25B1/04
CPCC25B1/04C25B11/04Y02E60/36
Inventor 涂宝峰程谟杰
Owner DALIAN INST OF CHEM PHYSICS CHINESE ACAD OF SCI