Synthetic method of 3-ethoxy-4-decoxyaniline as intermediate of decoquinate
A technology of decyloxyaniline and its synthesis method, which is applied in the field of chemical synthesis, can solve the problems such as side reactions are not easy to control, and achieve the effects of low raw material cost, simple and easy process, and low equipment requirements
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Embodiment 1
[0037] Add 200 grams of DMF to a 500 ml flask, add 70 grams of anhydrous potassium carbonate, 50 grams of o-hydroxyphenethyl ether, and 90 grams of bromodecane respectively, stir and heat up to 70±5°C, and the reaction and heat preservation take 4 to 8 hours.
[0038] Distill under reduced pressure (-0.09MPa, less than 90°C) until the material in the bottle is viscous, add 150 grams of water and 6 grams of potassium bromide, adjust the pH to 9-10 with 30% sodium hydroxide, add tetrabutylammonium bromide ( or benzyltriethylammonium chloride) 1 g. Stir for half an hour.
[0039] Install air guide tube and constant pressure dropping funnel, fill 60 grams of 30% sodium hydroxide in the funnel, temperature in the stirring bottle is 30-40 ℃, pass into chlorine gas, tail gas export and absorb with sodium hydroxide. Sodium hydroxide is added dropwise for 3-6 hours, the rate of chlorine flow is synchronized with the rate of dripping sodium hydroxide, and the pH is controlled at 8-10. ...
Embodiment 2
[0043] Add 200 grams of DMF to a 500 ml flask, add 70 grams of anhydrous potassium carbonate, 50 grams of o-hydroxyphenethyl ether, and 95 grams of decane bromide, stir and heat up to 70±5°C, and the reaction and heat preservation take 4 to 8 hours.
[0044] Distill under reduced pressure (-0.09MPa, less than 90°C) until the material in the bottle is viscous, add 150 grams of water and 5 grams of potassium bromide, adjust the pH to 9-10 with 30% sodium hydroxide, add tetrabutylammonium bromide ( or benzyltriethylammonium chloride) 1 g. Stir for half an hour.
[0045] Install air guide tube and constant pressure dropping funnel, fill 60 grams of 30% sodium hydroxide in the funnel, temperature in the stirring bottle is 30-40 ℃, pass into chlorine gas, tail gas export and absorb with sodium hydroxide. Sodium hydroxide is added dropwise for 3-6 hours, the rate of chlorine flow is synchronized with the rate of dripping sodium hydroxide, and the pH is controlled at 8-10.
[0046] Af...
Embodiment 3
[0049] Add 200 grams of DMF to a 500 ml flask, add 70 grams of anhydrous potassium carbonate, 50 grams of o-hydroxyphenethyl ether, and 100 grams of bromodecane respectively, stir and heat up to 70±5°C, and the reaction and heat preservation take 4 to 8 hours.
[0050] Distill under reduced pressure (-0.09MPa, less than 90°C) until the material in the bottle is viscous, add 150 grams of water and 5 grams of potassium bromide, adjust the pH to 9-10 with 30% sodium hydroxide, add tetrabutylammonium bromide ( or benzyltriethylammonium chloride) 1 g. Stir for half an hour.
[0051] Install air guide tube and constant pressure dropping funnel, fill 60 grams of 30% sodium hydroxide in the funnel, temperature in the stirring bottle is 30-40 ℃, pass into chlorine gas, tail gas export and absorb with sodium hydroxide. Sodium hydroxide is added dropwise for 3-6 hours, the rate of chlorine flow is synchronized with the rate of dripping sodium hydroxide, and the pH is controlled at 8-10....
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