Novel 4-aminopyridine and 6-aminopyrimidine carboxylates as herbicides
A C1-C6, alkyl technology, applied in the field of new 4-aminopyridine and 6-aminopyrimidine carboxylates as herbicides, can solve problems affecting crop yields, etc.
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[0188] Preparation method of compound
[0189] Exemplary methods of synthetic (I) compounds are provided below.
[0190] The 3,5-di-substituted-4-amino-6- (optionally substituted phenyl or pyridyl) pyridine-2-formic acid can be prepared in a variety of ways. As shown in Scheme I, the 4-amino-6-chlorine-pyridin-2-formate of formula (II) can be coupled to the suzuki of boric acid or ester, such as potassium fluoride and catalyst such as double (three Phenylphosphine) - Palladium (II) of Palladium (II) in the polaromy solvent mixture such as acetonitrile - water in, for example, 110 ° C, for example, converted into a 4-amino group of formula (III) in a microwave reactor- 6- Substituted - pyridine-2-formate, wherein Ar is as defined herein (reactive A 1 ). The 4-amino-6-substituted-pyridine-2-formate of the formula (III) can be converted to the formula (IV) by reaction with the iodinated reagent such as methanol, such as methanol, such as methanol, such as methanol. 5-iodo-4-amino-6-s...
Embodiment 1
[0231] Example 1: Preparation 4-amino-3,6-dichloro - pyridin-2-formate (head a)
[0232]
[0233] For the fabrication of Fields et al., WO 2001051468 A1 is prepared.
Embodiment 2
[0234] Example 2: Preparation 4-amino-3,6-dichloro-5-fluorine-pyridine-2-formate (head B)
[0235]
[0236] For example, Tetrahedron Letters 2010, 51, 79-81 is prepared in Tetrahedron Letters 2010, 51, 79-81.
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