Compounds containing acridinium esters and methods of using same for chemiluminescence-based monochromatic sequencing
A technology of compounds and compositions, applied in the field of single-color nucleic acid sequencing, can solve problems such as limited value of chemiluminescence
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[0082] Embodiment 1: the synthesis containing acridinium ester compound
[0083] General procedure for the preparation of compound 3:
[0084]
[0085] To a 250 mL flask was added 3-bromoanisole (5.0 g), 3-methoxyaniline (4.0 g), palladium acetate (0.21 g), 2,2'-bis(diphenylphosphino)-1, 1'-Binaphthyl (BINAP; 0.8 g), cesium carbonate (9.6 g) and toluene (100 mL). The mixture was degassed for 5 minutes, then refluxed under argon for 3 days. Water was added to the cooled reaction mixture, followed by extraction with ethyl acetate (EtOAc). The extract was washed with water and washed with anhydrous sodium sulfate (Na 2 SO 4 )dry. The crude product was purified by silica gel column chromatography to give compound 3.
[0086] General procedure for the preparation of compound 4:
[0087]
[0088] Compound 3 (2.5 g) in toluene (60 mL) was slowly added to a solution of oxalyl chloride (3.0 mL) in toluene (100 mL) using an additional funnel. After the addition was complete,...
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